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Here, we report a bioinspired twisted brick\u2013mortar composite that integrates a carbon\u2010nanotube\u2010reinforced photopolymer framework with a mechanically active shear\u2010stiffening gel mortar. The continuously twisted brick architecture redistributes stress waves and guides crack deflection, whereas reversible interfacial hydrogen bonding and dynamic boron\u2013oxygen crosslinking enable rate\u2010dependent molecular dissipation. This structural\u2013molecular coupling provides efficient impact protection, delivering a low energy transfer rate of 7.38% under high\u2010strain\u2010rate compression and reducing the residual impact force from 20\u00b0C to 100\u00b0C. The carbon\u2010nanotube\u2010containing framework further provides photothermal responsiveness, allowing reversible stifhefness modulation, adaptive force buffering, and shape recovery after localized high\u2010speed impacts. Together, these results establish a bioinspired twisted brick\u2013mortar design strategy for adaptive thermo\u2010mechanical impact protection.<\/jats:p>","DOI":"10.1002\/adma.75226","type":"journal-article","created":{"date-parts":[[2026,10,1]],"date-time":"2026-10-01T07:23:43Z","timestamp":1790839423000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Bioinspired Twisted Brick\u2013Mortar Composites for Adaptive Thermo\u2010Mechanical Impact Protection"],"prefix":"10.1002","author":[{"given":"Zimu","family":"Li","sequence":"first","affiliation":[{"name":"Department of Modern Mechanics University of Science and Technology of China  Hefei Anhui P. R. 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