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Herein, we develop a Hub\u2010Driven Ring Fusion (HDRF) strategy for constructing extended metallic topologies beyond discrete motifs. Guided by this strategy, we synthesize an atomically precise Pd\n                    <jats:sub>11<\/jats:sub>\n                    nanocluster featuring a rare fused tri\u2010pentagonal metal\u2010ring network. Magnetic shielding and nucleus\u2010independent chemical shift (NICS) analyses reveal pronounced spatial anisotropy and discontinuous shielding distributions, indicating a breakdown of global electronic coherence and the formation of partitioned electronic domains across fused rings. These \u201ctopology\u2010induced electronic domains\u201d connectivity\u2010governed electronic fragmentation, rather than uniform delocalization, defines the intrinsic electronic landscape of the cluster and clarifies that it is not merely a simple size expansion of Pd\n                    <jats:sub>5<\/jats:sub>\n                    . Pd\n                    <jats:sub>11<\/jats:sub>\n                    exhibits significantly enhanced performance in the electrocatalytic hydrogenation of nitrobenzene, achieving 98.1% conversion, 97.4% aniline yield, and 99.3% selectivity, outperforming Pd\n                    <jats:sub>5<\/jats:sub>\n                    and Pd\n                    <jats:sub>8<\/jats:sub>\n                    clusters. Density functional theory (DFT) calculations further demonstrate that the fused tri\u2010pentagonal topology optimizes electron distribution, enhances interfacial reactivity, and lowers the overall reaction barrier, providing a mechanistic basis for the observed catalytic enhancement.\n                  <\/jats:p>","DOI":"10.1002\/adma.75240","type":"journal-article","created":{"date-parts":[[2026,10,7]],"date-time":"2026-10-07T06:28:53Z","timestamp":1791354533000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Toward Two\u2010Dimensional Metallic Topologies in Atomically Precise Nanoclusters"],"prefix":"10.1002","author":[{"given":"Xi","family":"Chen","sequence":"first","affiliation":[{"name":"Key Laboratory of Materials Physics Anhui Key Laboratory of Nanomaterials and Nanotechnology CAS Center for Excellence in Nanoscience Institute of Solid State Physics HFIPS Chinese Academy of Sciences  Hefei 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