{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,10]],"date-time":"2026-10-10T04:48:49Z","timestamp":1791607729137,"version":"4.3.4"},"reference-count":56,"publisher":"Wiley","license":[{"start":{"date-parts":[[2026,10,9]],"date-time":"2026-10-09T00:00:00Z","timestamp":1791504000000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/onlinelibrary.wiley.com\/termsAndConditions#vor"},{"start":{"date-parts":[[2026,10,9]],"date-time":"2026-10-09T00:00:00Z","timestamp":1791504000000},"content-version":"tdm","delay-in-days":0,"URL":"http:\/\/doi.wiley.com\/10.1002\/tdm_license_1.1"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["52171014"],"award-info":[{"award-number":["52171014"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100000781","name":"European Research Council","doi-asserted-by":"publisher","award":["856538"],"award-info":[{"award-number":["856538"]}],"id":[{"id":"10.13039\/501100000781","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100000781","name":"European Research Council","doi-asserted-by":"publisher","award":["3D MAGiC"],"award-info":[{"award-number":["3D MAGiC"]}],"id":[{"id":"10.13039\/501100000781","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["advanced.onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["Advanced Materials"],"abstract":"ABSTRACT<\/jats:title>\n \n Sulfur is a promising high\u2010capacity cathode but suffers from sluggish redox kinetics and severe side reactions in aqueous electrolytes. We introduce pnictogen chalcohalide Bi\n 12.67<\/jats:sub>\n S\n 18<\/jats:sub>\n Br\n 2<\/jats:sub>\n nanorods (abbreviated as Bi\u2010S\u2010Br) as a multifunctional cathode material that functions as a sulfur\/bismuth reservoir and a catalytic redox mediator (RM). By integrating a trace amount of iodide electrolyte additive, we demonstrate a potential pathway, featuring several redox couples with gradient potentials: I\n 0<\/jats:sup>\n \/I\n \u2212<\/jats:sup>\n (0.530\u00a0V, RM1) > Bi\n 3+<\/jats:sup>\n \/Bi\n 0<\/jats:sup>\n (0.308\u00a0V, RM2) > S\n 0<\/jats:sup>\n \/S\n 2\u2212<\/jats:sup>\n (0.144\u00a0V vs. standard hydrogen electrode), whose stepwise dual mediation accelerates sulfur redox kinetics. The sulfurphilic Bi\u2010S\u2010Br nanorods also strengthen surface Bi\u2013S interfacial interactions, thus localizing active species and suppressing sulfur disproportionation. As a result, Zn||Bi\u2010S\u2010Br cells exhibit synergistic discharge plateaus at 0.66 and 0.59\u00a0V and deliver a high specific capacity of 792 mAh g\n Bi\u2010S\u2010Br<\/jats:sub>\n \u22121<\/jats:sup>\n at 0.4 A g\n \u22121<\/jats:sup>\n , with an energy density of 488.2\u00a0Wh kg\n \u22121<\/jats:sup>\n and a power density of 244.1\u00a0W kg\n \u22121<\/jats:sup>\n , normalized to the Bi\u2010S\u2010Br mass. The practical Zn||Bi\u2010S\u2010Br pouch cell configuration sustains 250 cycles at 0.8\u00a0mA cm\n \u22122<\/jats:sup>\n with capacity retention of 70.1%. This study elucidated the successive redox mediation strategy for enhanced sulfur redox kinetics, offering a new design principle for high\u2010performance aqueous energy storage systems.\n <\/jats:p>","DOI":"10.1002\/adma.75303","type":"journal-article","created":{"date-parts":[[2026,10,10]],"date-time":"2026-10-10T03:52:16Z","timestamp":1791604336000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Successive Redox Mediation Supported by Pnictogen Chalcohalide Enables High\u2010Performance Zinc\u2013Sulfur Batteries"],"prefix":"10.1002","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-9165-758X","authenticated-orcid":false,"given":"Shixun","family":"Wang","sequence":"first","affiliation":[{"name":"Department of Mechanical Engineering The University of Hong Kong Hong Kong SAR P. R. 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China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhuo","family":"Li","sequence":"additional","affiliation":[{"name":"Department of Materials Science and Engineering City University of Hong Kong Hong Kong SAR P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shimei","family":"Li","sequence":"additional","affiliation":[{"name":"Department of Mechanical Engineering The University of Hong Kong Hong Kong SAR P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shaoce","family":"Zhang","sequence":"additional","affiliation":[{"name":"Department of Mechanical Engineering The University of Hong Kong Hong Kong SAR P. R. 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