{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,7]],"date-time":"2026-10-07T08:55:41Z","timestamp":1791363341292,"version":"4.3.1"},"reference-count":49,"publisher":"Wiley","license":[{"start":{"date-parts":[[2026,10,7]],"date-time":"2026-10-07T00:00:00Z","timestamp":1791331200000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/onlinelibrary.wiley.com\/termsAndConditions#vor"},{"start":{"date-parts":[[2026,10,7]],"date-time":"2026-10-07T00:00:00Z","timestamp":1791331200000},"content-version":"tdm","delay-in-days":0,"URL":"http:\/\/doi.wiley.com\/10.1002\/tdm_license_1.1"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["22309112"],"award-info":[{"award-number":["22309112"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["22678361"],"award-info":[{"award-number":["22678361"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100013105","name":"Shanghai Rising-Star Program","doi-asserted-by":"publisher","award":["22QA1409000"],"award-info":[{"award-number":["22QA1409000"]}],"id":[{"id":"10.13039\/501100013105","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["advanced.onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["Advanced Materials"],"abstract":"<jats:title>ABSTRACT<\/jats:title>\n                  <jats:p>\n                    Self\u2010assembled monolayers (SAMs) containing carbazole and phosphonic acid groups have emerged as effective hole\u2010transport layers (HTLs) for high\u2010performance inverted perovskite solar cells (PSCs). However, the intrinsic aggregation tendency of SAM molecules often compromises interfacial uniformity, inducing non\u2010radiative recombination and limiting device efficiency and stability. Here, we report a synergistically assembled chemically heterogeneous (SACH) interfacial layer constructed by integrating [4\u2010(3,6\u2010dimethyl\u20109H\u2010carbazol\u20109\u2010yl)butyl]phosphonic acid (Me\u20104PACz) with carbazole\u20109\u2010ethanol (CE). In this strategy, CE promotes favorable heteromolecular \u03c0\u2010associated and dispersion interactions with Me\u20104PACz, thereby moderating excessive Me\u20104PACz self\u2010association, improving interfacial uniformity, and enhancing charge extraction. Meanwhile, the hydroxyl group of CE supports an O\u2500H\u00b7\u00b7\u00b7I\n                    <jats:sup>\u2212<\/jats:sup>\n                    interaction with perovskite, contributing to interfacial defect passivation and suppressed buried\u2010interface recombination. As a result, devices employing the SACH layer achieve a PCE of 27.06% (certified 26.86%). Under maximum power point tracking in ambient air at 65\u00b0C, encapsulated SACH\u2010based devices retained 88.6% of their initial efficiency after 500 h. Large\u2010area perovskite modules (30 \u00d7 30 cm\n                    <jats:sup>2<\/jats:sup>\n                    ) further demonstrate promising performance with an efficiency of 21.90%, highlighting the broad applicability of this cooperative interfacial design for scalable perovskite photovoltaics.\n                  <\/jats:p>","DOI":"10.1002\/adma.75318","type":"journal-article","created":{"date-parts":[[2026,10,7]],"date-time":"2026-10-07T08:46:03Z","timestamp":1791362763000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Cooperative Assembly Drives Buried Interface Engineering for Efficient Inverted Perovskite Solar Cells"],"prefix":"10.1002","author":[{"given":"Ranran","family":"Xu","sequence":"first","affiliation":[{"name":"School of Chemistry and Chemical Engineering Southeast University  Nanjing China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0002-9502-0460","authenticated-orcid":false,"given":"Ni","family":"Zhang","sequence":"additional","affiliation":[{"name":"School of Environmental Science and Engineering Frontiers Science Center for Transformative Molecules State Key Laboratory of Green Papermaking and Resource Recycling Shanghai Jiao Tong University  Shanghai China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0002-9859-9260","authenticated-orcid":false,"given":"Shengnan","family":"Wang","sequence":"additional","affiliation":[{"name":"School of Chemistry and Chemical Engineering Southeast University  Nanjing China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Fengqiao","family":"Xu","sequence":"additional","affiliation":[{"name":"School of Chemistry and Chemical Engineering Southeast University  Nanjing China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0008-2909-9792","authenticated-orcid":false,"given":"Weidong","family":"Lin","sequence":"additional","affiliation":[{"name":"School of Chemical and Environmental Engineering Shanghai Institute of Technology  Shanghai China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ruoting","family":"Liu","sequence":"additional","affiliation":[{"name":"School of Chemistry and Chemical Engineering Southeast University  Nanjing China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Lu","family":"Pan","sequence":"additional","affiliation":[{"name":"School of Chemistry and Chemical Engineering Southeast University  Nanjing China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8663-9993","authenticated-orcid":false,"given":"Yixin","family":"Zhao","sequence":"additional","affiliation":[{"name":"School of Environmental Science and Engineering Frontiers Science Center for Transformative Molecules State Key Laboratory of Green Papermaking and Resource Recycling Shanghai Jiao Tong University  Shanghai China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhixiao","family":"Qin","sequence":"additional","affiliation":[{"name":"Shanghai Pvsktech Co., Ltd.  Shanghai China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8224-5057","authenticated-orcid":false,"given":"Yongbing","family":"Lou","sequence":"additional","affiliation":[{"name":"School of Chemistry and Chemical Engineering Southeast University  Nanjing China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-4012-2785","authenticated-orcid":false,"given":"Taiyang","family":"Zhang","sequence":"additional","affiliation":[{"name":"School of Chemical and Environmental Engineering Shanghai Institute of Technology  Shanghai China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2026,10,7]]},"reference":[{"key":"e_1_2_8_2_1","doi-asserted-by":"crossref","DOI":"10.1016\/j.nanoen.2020.105400","article-title":"Perovskite\/Perovskite Planar Tandem Solar Cells: A Comprehensive Guideline for Reaching Energy Conversion Efficiency Beyond 30%","volume":"79","author":"Hossain M. 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Interfaces"},{"key":"e_1_2_8_26_1","doi-asserted-by":"crossref","first-page":"3860","DOI":"10.1021\/acsenergylett.3c01385","article-title":"Resolving the Hydrophobicity of the Me\u20104PACz Hole Transport Layer for Inverted Perovskite Solar Cells with Efficiency >20%","volume":"8","author":"Hossain K.","year":"2023","journal-title":"ACS Energy Letters"},{"key":"e_1_2_8_27_1","doi-asserted-by":"crossref","first-page":"818","DOI":"10.1038\/s41560-026-02014-9","article-title":"Molecular\u2010Templated Pre\u2010Assembly of Self\u2010Assembled Monolayer for Perovskite Solar Cells and Modules with Improved Reverse\u2010Bias Stability","volume":"11","author":"Wang X.","year":"2026","journal-title":"Nature Energy"},{"key":"e_1_2_8_28_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467\u2010026\u201076266\u20100"},{"key":"e_1_2_8_29_1","doi-asserted-by":"crossref","DOI":"10.1002\/adma.73306","article-title":"Molecular Polarization\u2010Driven Synergistic Interface Engineering for High\u2010Performance Perovskite Solar Cells","volume":"38","author":"Wang Y.","year":"2026","journal-title":"Advanced Materials"},{"key":"e_1_2_8_30_1","doi-asserted-by":"crossref","DOI":"10.1002\/adfm.202417575","article-title":"Improving Buried Interface Contact for Inverted Perovskite Solar Cells via Dual Modification Strategy","volume":"35","author":"Zhang Y.","year":"2024","journal-title":"Advanced Functional Materials"},{"key":"e_1_2_8_31_1","doi-asserted-by":"crossref","DOI":"10.1002\/adma.202520251","article-title":"Multifunctional Conjugated Ligands Synergistically Optimize the Interface and Regulate Crystallization for High\u2010Performance 2D\/3D Perovskite Solar Cells","volume":"38","author":"Yang Y.","year":"2026","journal-title":"Advanced Materials"},{"key":"e_1_2_8_32_1","doi-asserted-by":"crossref","DOI":"10.1016\/j.joule.2026.102492","article-title":"Homogeneously Distributed Self\u2010Assembled Molecules for Efficient and Scalable Perovskite\/Silicon Tandem Solar 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