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While miniaturization is advancing, active manipulation remains limited by the difficulty of achieving simultaneous milliwatt\u2010scale visible light generation and high\u2010contrast modulation. Despite extensive efforts, the concurrent chip\u2010scale realization of nonlinear frequency conversion and fast temporal gating for high\u2010fidelity quantum control has remained elusive. Here, we demonstrate a monolithic thin\u2010film lithium niobate (TFLN) platform integrating periodically poled frequency conversion with GHz\u2010bandwidth electro\u2010optic (EO) switching. The device delivers off\u2010chip green\u2010light power exceeding 1\u00a0mW with an extinction ratio (ER) of 42.2\u00a0dB, enabling coherent spin control and time\u2010resolved lifetime measurements of individual nitrogen\u2010vacancy (NV) centers in diamond through nanosecond gating. System performance is validated through pulsed optically detected magnetic resonance (ODMR), Rabi oscillations, and Ramsey interference, supported by time\u2010tagged photon counting with nanosecond resolution. By unifying sufficient nonlinear light generation with high\u2010speed active manipulation, this platform establishes a scalable framework for the realization of high\u2010rate quantum communication\u00a0nodes.<\/jats:p>","DOI":"10.1002\/adma.75321","type":"journal-article","created":{"date-parts":[[2026,10,14]],"date-time":"2026-10-14T07:06:38Z","timestamp":1791961598000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Nonlinear Electro\u2010Optic Visible Photonic Circuits for Solid\u2010State Quantum Defects"],"prefix":"10.1002","author":[{"ORCID":"https:\/\/orcid.org\/0009-0003-7502-1420","authenticated-orcid":false,"given":"Yongchan","family":"Park","sequence":"first","affiliation":[{"name":"Center for Quantum Technology Korea Institute of Science and Technology (KIST) Seoul South Korea"},{"name":"School of Electrical Engineering Korea University Seoul South 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