{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,24]],"date-time":"2026-10-24T07:38:44Z","timestamp":1792827524602,"version":"4.5.0"},"reference-count":43,"publisher":"Wiley","license":[{"start":{"date-parts":[[2026,10,24]],"date-time":"2026-10-24T00:00:00Z","timestamp":1792800000000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/onlinelibrary.wiley.com\/termsAndConditions#vor"},{"start":{"date-parts":[[2026,10,24]],"date-time":"2026-10-24T00:00:00Z","timestamp":1792800000000},"content-version":"tdm","delay-in-days":0,"URL":"http:\/\/doi.wiley.com\/10.1002\/tdm_license_1.1"}],"funder":[{"DOI":"10.13039\/501100012166","name":"National Key Research and Development Program of China","doi-asserted-by":"publisher","award":["2021YFA1500800"],"award-info":[{"award-number":["2021YFA1500800"]}],"id":[{"id":"10.13039\/501100012166","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["22572142"],"award-info":[{"award-number":["22572142"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["advanced.onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["Advanced Materials"],"abstract":"<jats:title>ABSTRACT<\/jats:title>\n                  <jats:p>\n                    Despite significant progress in photocatalytic half\u2010reactions and photoelectrochemical water oxidation, achieving stable photocatalytic pure water splitting over Ta\n                    <jats:sub>3<\/jats:sub>\n                    N\n                    <jats:sub>5<\/jats:sub>\n                    remains a long\u2010standing challenge. Herein, the incompatibility of cocatalysts between alkaline photocatalytic water oxidation systems and pure water splitting is identified as a critical bottleneck, leading to serious N\n                    <jats:sub>2<\/jats:sub>\n                    generation through photocorrosion. To address this challenge, a highly dispersed RuCoO\n                    <jats:sub>x<\/jats:sub>\n                    cocatalyst is developed via a multi\u2010step incipient wetness impregnation strategy. The optimized Pt@Cr\n                    <jats:sub>2<\/jats:sub>\n                    O\n                    <jats:sub>3<\/jats:sub>\n                    \/Ta\n                    <jats:sub>3<\/jats:sub>\n                    N\n                    <jats:sub>5<\/jats:sub>\n                    \/RuCoO\n                    <jats:sub>x<\/jats:sub>\n                    achieves stoichiometric pure water splitting with an apparent quantum yield of 0.72% at 420\u00a0nm, representing the highest value reported for Ta\u2010based nitride\/oxynitride photocatalysts to date. Mechanistic studies reveal that an enhanced interfacial electric field facilitates hole extraction, while a reduced formation barrier of key intermediates accelerates surface reaction kinetics, thereby overcoming the long\u2010standing bottleneck in photocatalytic pure water splitting over Ta\n                    <jats:sub>3<\/jats:sub>\n                    N\n                    <jats:sub>5<\/jats:sub>\n                    . This work establishes cocatalyst compatibility as a key design consideration for stable photocatalytic pure water splitting and provides mechanistic insight for the rational design of advanced nitride and oxynitride photocatalysts.\n                  <\/jats:p>","DOI":"10.1002\/adma.75490","type":"journal-article","created":{"date-parts":[[2026,10,24]],"date-time":"2026-10-24T07:34:33Z","timestamp":1792827273000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Bridging the Gap Between Photocatalytic Water Oxidation Half\u2010Reaction and Stoichiometric Pure Water Splitting Over Ta\n                    <sub>3<\/sub>\n                    N\n                    <sub>5<\/sub>\n                    via Cocatalyst Engineering"],"prefix":"10.1002","author":[{"ORCID":"https:\/\/orcid.org\/0009-0001-5175-6911","authenticated-orcid":false,"given":"Jiwei","family":"Cui","sequence":"first","affiliation":[{"name":"Advanced Catalytic Materials Research Center School of Materials Science and Engineering State Key Laboratory of Precious Metal Functional Materials Tianjin University  Tianjin China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0007-7479-3700","authenticated-orcid":false,"given":"Chenhe","family":"Wu","sequence":"additional","affiliation":[{"name":"Advanced Catalytic Materials Research Center School of Materials Science and Engineering State Key Laboratory of Precious Metal Functional Materials Tianjin University  Tianjin China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0008-6958-7029","authenticated-orcid":false,"given":"Yanhui","family":"Sun","sequence":"additional","affiliation":[{"name":"Advanced Catalytic Materials Research Center School of Materials Science and Engineering State Key Laboratory of Precious Metal Functional Materials Tianjin University  Tianjin 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Materials Science and Engineering State Key Laboratory of Precious Metal Functional Materials Tianjin University  Tianjin China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0006-3967-1882","authenticated-orcid":false,"given":"Yiyuan","family":"Wang","sequence":"additional","affiliation":[{"name":"Advanced Catalytic Materials Research Center School of Materials Science and Engineering State Key Laboratory of Precious Metal Functional Materials Tianjin University  Tianjin China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-3837-6831","authenticated-orcid":false,"given":"Lequan","family":"Liu","sequence":"additional","affiliation":[{"name":"Advanced Catalytic Materials Research Center School of Materials Science and Engineering State Key Laboratory of Precious Metal Functional Materials Tianjin University  Tianjin China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jinhua","family":"Ye","sequence":"additional","affiliation":[{"name":"Advanced Catalytic Materials Research Center School of Materials Science and Engineering State Key Laboratory of Precious Metal Functional Materials Tianjin University  Tianjin China"},{"name":"International Center For Materials Nano Architectonics (WPI\u2010MANA) National Institute for Materials Science (NIMS)  Tsukuba Japan"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2026,10,24]]},"reference":[{"key":"e_1_2_8_2_1","doi-asserted-by":"crossref","first-page":"2109","DOI":"10.1039\/C8CS00542G","article-title":"Recent Developments in Heterogeneous Photocatalysts for Solar\u2010Driven Overall Water Splitting","volume":"48","author":"Wang Z.","year":"2019","journal-title":"Chemical Society 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