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By contrast, more attention should be paid for the methane oxidation and conversion, which can help the effective utilization of methane without emission. However, methane conversion and utilization under ambient conditions remains a challenge. Here, this study designs a Co\n                    <jats:sub>3<\/jats:sub>\n                    O\n                    <jats:sub>4<\/jats:sub>\n                    \/ZrO\n                    <jats:sub>2<\/jats:sub>\n                    nanocomposite for the electrochemical oxidation of methane gas using a carbonate electrolyte at room temperature. Co\n                    <jats:sub>3<\/jats:sub>\n                    O\n                    <jats:sub>4<\/jats:sub>\n                    activated the highly efficient oxidation of methane under mild electric energy with the help of carbonate as an oxidant, which is delivered by ZrO\n                    <jats:sub>2<\/jats:sub>\n                    . Based on the experimental results, acetaldehyde is the key intermediate product. Subsequent nucleophilic addition and free radical addition reactions accounted for the generation of 2\u2010propanol and 1\u2010propanol, respectively. Surprisingly, this work achieves a production efficiency of over 60% in the conversion of methane to produce these long\u2010term stable products. The as\u2010proposed regional electrochemical methane oxidation provides a new pathway for the synthesis of higher alcohols with high production efficiencies under ambient conditions.\n                  <\/jats:p>","DOI":"10.1002\/advs.201700379","type":"journal-article","created":{"date-parts":[[2017,9,11]],"date-time":"2017-09-11T03:08:48Z","timestamp":1505099328000},"source":"Crossref","is-referenced-by-count":106,"title":["Ultrahigh Electrocatalytic Conversion of Methane at Room Temperature"],"prefix":"10.1002","volume":"4","author":[{"given":"Ming","family":"Ma","sequence":"first","affiliation":[{"name":"Department of Chemical and Biomolecular Engineering Yonsei University  50 Yonsei\u2010ro Seodaemun\u2010gu Seoul 120\u2010749 Republic of Korea"},{"name":"SKKU Advanced Institute of Nano Technology (SAINT) Sungkyunkwan University  Chunchun\u2010dong Suwon 440\u2010746 Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Bing Jun","family":"Jin","sequence":"additional","affiliation":[{"name":"Department of Chemical and Biomolecular Engineering Yonsei University  50 Yonsei\u2010ro Seodaemun\u2010gu Seoul 120\u2010749 Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ping","family":"Li","sequence":"additional","affiliation":[{"name":"Department of Chemical and Biomolecular Engineering Yonsei University  50 Yonsei\u2010ro Seodaemun\u2010gu Seoul 120\u2010749 Republic of Korea"},{"name":"SKKU Advanced Institute of Nano Technology (SAINT) Sungkyunkwan University  Chunchun\u2010dong Suwon 440\u2010746 Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Myung Sun","family":"Jung","sequence":"additional","affiliation":[{"name":"Department of Chemical and Biomolecular Engineering Yonsei University  50 Yonsei\u2010ro Seodaemun\u2010gu Seoul 120\u2010749 Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jin Il","family":"Kim","sequence":"additional","affiliation":[{"name":"Department of Chemical and Biomolecular Engineering Yonsei University  50 Yonsei\u2010ro Seodaemun\u2010gu Seoul 120\u2010749 Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yoonjun","family":"Cho","sequence":"additional","affiliation":[{"name":"Department of Chemical and Biomolecular Engineering Yonsei University  50 Yonsei\u2010ro Seodaemun\u2010gu Seoul 120\u2010749 Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Sungsoon","family":"Kim","sequence":"additional","affiliation":[{"name":"Department of Chemical and Biomolecular Engineering Yonsei University  50 Yonsei\u2010ro Seodaemun\u2010gu Seoul 120\u2010749 Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jun Hyuk","family":"Moon","sequence":"additional","affiliation":[{"name":"Department of Chemical and Biomolecular Engineering Sogang University  1 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