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Here, environment\u2010friendly strategies for the separation, retreatment, and utilization of microplastics via electrocoagulation are investigated. The findings show that the flocs generated by forming Fe<jats:sub>3<\/jats:sub>O<jats:sub>4<\/jats:sub> on the surface of polyethylene (PE) particles are easily separated using a magnetic force with high efficiency of 98.4%. In the photodegradation of the obtained flocs, it is confirmed that Fe<jats:sub>3<\/jats:sub>O<jats:sub>4<\/jats:sub> shall be removed for the efficient generation of free radicals, leading to the highly efficient photolysis of PE. The removed Fe<jats:sub>3<\/jats:sub>O<jats:sub>4<\/jats:sub> can be recycled into iron\u2010oxalate compounds, which can be used in battery applications. In addition, it is suggested that heat treatment of Fe<jats:sub>3<\/jats:sub>O<jats:sub>4<\/jats:sub>\u2013PE flocs in an Ar atmosphere leads to forming Fe<jats:sub>3<\/jats:sub>O<jats:sub>4<\/jats:sub> core\u2013carbon shell nanoparticles, which show excellent performance as anodes in lithium\u2010ion batteries. The proposed composite exhibits an excellent capacity of 1123 mAh g<jats:sup>\u22121<\/jats:sup> at the current density of 0.5 A g<jats:sup>\u22121<\/jats:sup> after 600 cycles with a negative fading phenomenon. This study offers insight into a new paradigm of recyclable processes, from environmental issues such as microplastics to using energy materials.<\/jats:p>","DOI":"10.1002\/advs.202205675","type":"journal-article","created":{"date-parts":[[2023,1,16]],"date-time":"2023-01-16T21:40:26Z","timestamp":1673905226000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":16,"title":["Recycling Microplastics to Fabricate Anodes for Lithium\u2010Ion Batteries: From Removal of Environmental Troubles via Electrocoagulation to Useful Resources"],"prefix":"10.1002","volume":"10","author":[{"given":"Jinhee","family":"Lee","sequence":"first","affiliation":[{"name":"Department of Chemistry and Chemical Engineering Inha University  Incheon 22212 Republic of 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