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In this work, a buckled plumbene\u2010Au Kagome superstructure grown by depositing Au on Pb(111) is investigated. The superconducting gap monitored by temperature\u2010dependent scanning tunneling microscopy\/spectroscopy shows that the buckled plumbene\u2010Au Kagome superstructure not only has an enhanced <jats:italic>T<\/jats:italic><jats:sub>c<\/jats:sub> with respect to that of a monolayer Pb but also possesses a higher value than what owned by a bulk Pb substrate. By combining angle\u2010resolved photoemission spectroscopy with density functional theory, the monolayer Au\u2010intercalated low\u2010buckled plumbene sandwiched between the top Au Kagome layer and the bottom Pb(111) substrate is confirmed and the electron\u2013phonon coupling\u2010enhanced superconductivity is revealed. This work demonstrates that a buckled plumbene\u2010Au Kagome superstructure can enhance superconducting <jats:italic>T<\/jats:italic><jats:sub>c<\/jats:sub> and Rashba effect, effectively triggering the novel properties of a plumbene.<\/jats:p>","DOI":"10.1002\/advs.202300845","type":"journal-article","created":{"date-parts":[[2023,5,3]],"date-time":"2023-05-03T07:19:02Z","timestamp":1683098342000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":6,"title":["Enhanced Superconductivity and Rashba Effect in a Buckled Plumbene\u2010Au Kagome Superstructure"],"prefix":"10.1002","volume":"10","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-5544-3381","authenticated-orcid":false,"given":"Wan\u2010Hsin","family":"Chen","sequence":"first","affiliation":[{"name":"Department of Electrophysics National Yang Ming Chiao Tung University  Hsinchu 300 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