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However, due to safety concerns and limitations in <jats:italic>operando<\/jats:italic> characterization at high state\u2010of\u2010charges (SoCs), the fundamental understanding of stress\u2010driven ISCs under high SOC situations (above 30%) is still lacking. In this study, combined post\u2010mortem characterization and multiphysics modeling is employed to clarify the evolution of ISC modes in LIBs with high SOCs. These findings reveal that the triggered ISC mode is SOC\u2010dependent, with the Al current collector (Al)\u2010Anode coating (An) mode dominant in high SOC situations. Experimentally obtained ISC resistance for the specified ISC mode is then assigned to the corresponding ISC region in the established multiphysics model, allowing for accurate coupling of the electromechanical relationship and prediction of mechanical\u2010electrical\u2010thermal responses of the LIB. Finally, a simple yet effective approach is proposed for avoiding the Al\u2010An mode after battery fractures, achieved through surface notches on electrodes. Results discover novel phenomena for ISC in high SOC cells and reveal the underlying mechanisms, highlighting the importance and potential of battery structural design for developing next\u2010generation robust batteries.<\/jats:p>","DOI":"10.1002\/advs.202302496","type":"journal-article","created":{"date-parts":[[2023,8,9]],"date-time":"2023-08-09T04:23:15Z","timestamp":1691554995000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":39,"title":["Understanding of Stress\u2010Driven Internal Short Circuit Mechanisms in Lithium\u2010Ion Batteries with High SOCs"],"prefix":"10.1002","volume":"10","author":[{"given":"Xudong","family":"Duan","sequence":"first","affiliation":[{"name":"Department of Automotive Engineering School of Transportation Science and Engineering Beihang University  Beijing 100191 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