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In this study, by finding an autonomous phase separating ability of fungal mycelium, a new material fabrication approach is introduced that leverages such biological metabolism\u2010driven, mycelial growth\u2010induced phase separation to bypass high\u2010energy cost and labor\u2010intensive synthetic methods. The resulting self\u2010regenerative composites, featuring an entangled network structure of mycelium and assembled organic polymers, exhibit remarkable self\u2010healing properties, being capable of reversing complete separation and restoring \u224890% of the original strength. These composites further show exceptional mechanical strength, with a high specific strength of 8.15\u00a0MPa\u00a0g.cm\n                    <jats:sup>\u22123<\/jats:sup>\n                    , and low water absorption properties (\u224833% after 15 days of immersion). This approach spearheads the development of state\u2010of\u2010the\u2010art living composites, which directly utilize bioactive materials to \u201cself\u2010grow\u201d into materials endowed with exceptional mechanical and functional properties.\n                  <\/jats:p>","DOI":"10.1002\/advs.202309370","type":"journal-article","created":{"date-parts":[[2024,3,13]],"date-time":"2024-03-13T07:50:32Z","timestamp":1710316232000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":20,"title":["Fabrication of Living Entangled Network Composites Enabled by Mycelium"],"prefix":"10.1002","volume":"11","author":[{"given":"Hao","family":"Wang","sequence":"first","affiliation":[{"name":"Department of Mechanical Engineering City University of Hong Kong  Kowloon Hong Kong"},{"name":"Shaping Matter Lab Faculty of Aerospace Engineering Delft University of Technology  Delft 2629 HS Netherlands"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jie","family":"Tao","sequence":"additional","affiliation":[{"name":"School of Materials Science and Technology Nanjing University of Aeronautics and Astronautics  Nanjing Jiangsu 211106 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhangyu","family":"Wu","sequence":"additional","affiliation":[{"name":"School of Materials Science and Engineering Southeast University  Nanjing 211189 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Kathrin","family":"Weiland","sequence":"additional","affiliation":[{"name":"Shaping Matter Lab Faculty of Aerospace Engineering Delft University of Technology  Delft 2629 HS Netherlands"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zuankai","family":"Wang","sequence":"additional","affiliation":[{"name":"Department of Mechanical Engineering The Hong Kong Polytechnic University  Hung Hom Kowloon Hong Kong"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Kunal","family":"Masania","sequence":"additional","affiliation":[{"name":"Shaping Matter Lab Faculty of Aerospace Engineering Delft University of Technology  Delft 2629 HS Netherlands"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-6927-9247","authenticated-orcid":false,"given":"Bin","family":"Wang","sequence":"additional","affiliation":[{"name":"Department of Mechanical Engineering City University of Hong Kong  Kowloon Hong Kong"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2024,3,13]]},"reference":[{"key":"e_1_2_9_1_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.scitotenv.2021.146695"},{"key":"e_1_2_9_2_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.envpol.2019.01.097"},{"key":"e_1_2_9_3_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41563-023-01628-8"},{"key":"e_1_2_9_4_1","volume":"30","author":"Peter Q. 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