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However, current LIG\u2010based TENG commonly rely on polymer films, e.g., polyimide (PI) as both friction material and carbon precursor of electrodes, which limit the structural diversity and performance escalation due to its incapability of folding and creasing. Using specialized PI paper composed of randomly distributed PI fibers to substantially enhance its foldability, this work creates a new type of TENG, which are structurally foldable and stackable, and performance tailorable. First, by systematically investigating the laser power\u2010regulated performance of single\u2010unit TENG, the open\u2010circuit voltage can be effectively improved. By further exploiting the folding process, multiple TENG units can be assembled together to form multi\u2010layered structures to continuously expand the open\u2010circuit voltage from 5.3 to 34.4\u00a0V\u00a0cm<jats:sup>\u22122<\/jats:sup>, as the increase of friction units from 1 to 16. Last, by fully utilizing the unique structure and performance, representative energy\u2010harvesting and smart\u2010sensing applications are demonstrated, including a smart shoe to recognize running motions and power LEDs, a smart leaf to power a thermometer by wind, a matrix sensor to recognize writing trajectories, as well as a smart glove to recognize different objects.<\/jats:p>","DOI":"10.1002\/advs.202310017","type":"journal-article","created":{"date-parts":[[2024,5,15]],"date-time":"2024-05-15T05:49:30Z","timestamp":1715752170000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":39,"title":["Structure\u2010Foldable and Performance\u2010Tailorable PI Paper\u2010Based Triboelectric Nanogenerators Processed and Controlled by Laser\u2010Induced Graphene"],"prefix":"10.1002","volume":"11","author":[{"given":"Weixiong","family":"Yang","sequence":"first","affiliation":[{"name":"School of Mechanical Engineering &amp; Automation Beihang University  No. 37 Xueyuan Road Beijing 100191 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Mingguang","family":"Han","sequence":"additional","affiliation":[{"name":"School of Mechanical Engineering &amp; 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