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It is an urgent need to develop effective underoil adhesives. However, realizing underoil adhesion is even harder than those underwater, due to the stubborn attachment of a highly viscous oil layer on target surface. Here, inspired by endocytosis, a tough gel tape composed of zwitterionic polymer network and zwitterionic surfactants is developed. The amphiphilic surfactants can form micelle to capture the oil droplets and transport them from the interface to gel via electrostatic attraction of polymer backbone, mimicking the endocytosis and achieving robust underoil adhesion. Benefiting from the oil\u2010resistance of polymer backbone, the gel further realizes a combination of i) long\u2010term adhesion with high durability, ii) repeated adhesion in oil, and iii) renewable adhesion efficiency after exhausted use. The tape exhibits an ultra\u2010high adhesive toughness of 2446.86 J m<jats:sup>\u22122<\/jats:sup> to stainless steel in silicone oil after 30 days' oil\u2010exposure; such value of adhesive toughness surpasses many of those achieved in underwater adhesion and is greater than underoil adhesion performance of commercial tape. The strategy illustrated here will motivate the design of sustainable and efficient adhesives for wet environments.<\/jats:p>","DOI":"10.1002\/advs.202407501","type":"journal-article","created":{"date-parts":[[2024,9,9]],"date-time":"2024-09-09T07:43:58Z","timestamp":1725867838000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":19,"title":["Endocytosis\u2010Inspired Zwitterionic Gel Tape for High\u2010Efficient and Sustainable Underoil Adhesion"],"prefix":"10.1002","volume":"11","author":[{"given":"Yueman","family":"Tang","sequence":"first","affiliation":[{"name":"College of Materials Science &amp; Engineering Zhejiang University of Technology  Hangzhou 310014 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Mengjie","family":"Si","sequence":"additional","affiliation":[{"name":"College of Materials Science &amp; Engineering Zhejiang University of Technology  Hangzhou 310014 P. R. 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