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In this work, a series of hexabenzocoronene\u2010based single\u2010molecule junctions are successfully constructed, and their temperature\u2010dependent charge transport properties are studied. It is found that rotational vibrations of both benzene and hexabenzocoronene rings are sequentially excited as the temperature increases, and the electron\u2010vibration coupling enhances charge tunneling. In addition, the transition temperature between distinct vibration\u2010assisted tunneling modes and the activation energies show\u00a0strong correlations with the molecular vibration frequency and molecular length. This study unveils the distinct dual\u2010vibration\u2010assisted molecular tunneling mechanism, significantly enhancing the ability to precisely control molecular charge transport and develop functional molecular devices.<\/jats:p>","DOI":"10.1002\/advs.202408310","type":"journal-article","created":{"date-parts":[[2024,11,20]],"date-time":"2024-11-20T12:38:57Z","timestamp":1732106337000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":5,"title":["Dual\u2010Vibration\u2010Assisted Charge Transport Through Hexabenzocoronene in Single\u2010Molecule Junctions"],"prefix":"10.1002","volume":"12","author":[{"given":"Miao","family":"Zhang","sequence":"first","affiliation":[{"name":"Center of Single\u2010Molecule Sciences Institute of Modern Optics Frontiers Science Center for New Organic Matter Tianjin Key Laboratory of Micro\u2010Scale Optical Information Science and Technology College of Electronic Information and Optical Engineering Nankai University  38 Tongyan Road, Jinnan District Tianjin 300350 P. 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