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However, ion migration caused by high operating electric field remains a bottleneck limiting the long\u2010term stability of perovskite X\u2010ray detectors. Herein, by introducing multiple halogen interactions in lead\u2010free perovskites, stable X\u2010ray detection is successfully realized. Specifically, 0D polar bismuth halide perovskites (\n                    <jats:italic>R<\/jats:italic>\n                    \/\n                    <jats:italic>S<\/jats:italic>\n                    \u2010BPEA)\n                    <jats:sub>4<\/jats:sub>\n                    Bi\n                    <jats:sub>2<\/jats:sub>\n                    I\n                    <jats:sub>10<\/jats:sub>\n                    (\n                    <jats:bold>\n                      1\n                      <jats:italic>R<\/jats:italic>\n                    <\/jats:bold>\n                    \/\n                    <jats:bold>\n                      1\n                      <jats:italic>S<\/jats:italic>\n                    <\/jats:bold>\n                    ,\n                    <jats:italic>R<\/jats:italic>\n                    \/\n                    <jats:italic>S<\/jats:italic>\n                    \u2010BPEA =\n                    <jats:italic>R<\/jats:italic>\n                    \/\n                    <jats:italic>S<\/jats:italic>\n                    \u20101\u2010(4\u2010bromophenyl)ethylammonium) are designed by introducing Br\u2010substituted chiral organic cation BPEA, which exists with the molecular electrostatic forces between the Br atom and neighboring benzene ring and halogen interaction of Br\u00b7\u00b7\u00b7I. Notably, their introduction improves the activation energy of ion migration, which makes the dark current drift of the X\u2010ray detector as low as 3.25 \u00d7 10\n                    <jats:sup>\u22128<\/jats:sup>\n                    nA cm\n                    <jats:sup>\u22121<\/jats:sup>\n                    s\n                    <jats:sup>\u22121<\/jats:sup>\n                    V\n                    <jats:sup>\u22121<\/jats:sup>\n                    at 2500 V cm\n                    <jats:sup>\u22121<\/jats:sup>\n                    . Furthermore, the excellent operational stability under prolonged X\u2010ray irradiation and unchanged device sensitivity after 90 days of exposure to air, further demonstrates the improved stability of perovskites. Meanwhile, the chiral\u2010polar characteristic of the\n                    <jats:bold>\n                      1\n                      <jats:italic>R<\/jats:italic>\n                    <\/jats:bold>\n                    \/\n                    <jats:bold>\n                      1\n                      <jats:italic>S<\/jats:italic>\n                    <\/jats:bold>\n                    gives them potential for self\u2010powered detection, with a low detection limit of 183 nGy s\n                    <jats:sup>\u22121<\/jats:sup>\n                    at zero bias for single\u2010crystal devices. This study opens new avenues for the future development of \u201cgreen\u201d, highly stable, self\u2010powered radiation detectors.\n                  <\/jats:p>","DOI":"10.1002\/advs.202412504","type":"journal-article","created":{"date-parts":[[2025,4,4]],"date-time":"2025-04-04T22:06:41Z","timestamp":1743804401000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":16,"title":["Multiple Interactions in Polar Lead\u2010Free Perovskites toward Highly Stable X\u2010Ray Detection"],"prefix":"10.1002","volume":"12","author":[{"given":"Chang","family":"Qu","sequence":"first","affiliation":[{"name":"State Key Laboratory of Functional Crystals and Devices Fujian Institute of Research on the Structure of Matter Chinese Academy of Sciences  Fuzhou Fujian 350002 P. R. China"},{"name":"College of Chemistry and Materials Science Fujian Normal University  Fuzhou 350007 P. R. 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