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Here, a TMO with all these features is reported, existing as an interfacial phase in the 4\n                    <jats:italic>d<\/jats:italic>\n                    Ca\n                    <jats:sub>0.5<\/jats:sub>\n                    Sr\n                    <jats:sub>0.5<\/jats:sub>\n                    RuO\n                    <jats:sub>3<\/jats:sub>\n                    layer sandwiched by two LaMnO\n                    <jats:sub>3<\/jats:sub>\n                    layers. This phase is well conductive and ferromagnetic in a wide temperature range, with the highest Curie temperature of \u2248275\u00a0K among the 4\n                    <jats:italic>d<\/jats:italic>\n                    \/5\n                    <jats:italic>d<\/jats:italic>\n                    \u2010TMOs. Particularly, this interfacial phase shows a considerably improved saturation magnetization (\u22482\u00a0\n                    <jats:italic>\u00b5<\/jats:italic>\n                    <jats:sub>B<\/jats:sub>\n                    \/Ru, twice that of the bulk counterpart), and a greatly reduced coercive force. All these features are highly desired by the application of spin\u2010orbit torque. Due to the presence of strong spin\u2010orbit coupling, such a Ca\n                    <jats:sub>0.5<\/jats:sub>\n                    Sr\n                    <jats:sub>0.5<\/jats:sub>\n                    RuO\n                    <jats:sub>3<\/jats:sub>\n                    interfacial phase exhibits a significantly larger anomalous Hall conductivity than the typical 3\n                    <jats:italic>d<\/jats:italic>\n                    oxide ferromagnet La\n                    <jats:sub>2\/3<\/jats:sub>\n                    Sr\n                    <jats:sub>1\/3<\/jats:sub>\n                    MnO\n                    <jats:sub>3<\/jats:sub>\n                    near room temperature. Analyses based on the techniques of X\u2010ray magnetic circular dichroism, polarized\u2010neutron reflectometry, and scanning transmission electron microscopy reveal a magnetic exchange interaction between the interfacial phases of Ca\n                    <jats:sub>0.5<\/jats:sub>\n                    Sr\n                    <jats:sub>0.5<\/jats:sub>\n                    RuO\n                    <jats:sub>3<\/jats:sub>\n                    and LaMnO\n                    <jats:sub>3<\/jats:sub>\n                    and an obvious expansion of the interfacial Mn\u2500O\u2500Mn bond angle, stabilizing the high\u2010temperature ferromagnetic state of the CSRO\/LMO interface.\n                  <\/jats:p>","DOI":"10.1002\/advs.202502613","type":"journal-article","created":{"date-parts":[[2025,6,19]],"date-time":"2025-06-19T07:41:08Z","timestamp":1750318868000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Near Room\u2010Temperature Ferromagnetic Phase Achieved in 4\n                    <i>d<\/i>\n                    Ruthenate via Interfacial Ferrimagnetic Coupling and Octahedral Rotation Engineering"],"prefix":"10.1002","volume":"12","author":[{"given":"Mengqin","family":"Wang","sequence":"first","affiliation":[{"name":"Beijing National Laboratory for Condensed Matter Physics and Institute of Physics Chinese Academy of Sciences  Beijing 100190 China"},{"name":"School of Physical Sciences University of Chinese Academy of Sciences  Beijing 100049 China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Qinghua","family":"Zhang","sequence":"additional","affiliation":[{"name":"Beijing National Laboratory for Condensed Matter Physics and Institute of Physics Chinese Academy of Sciences  Beijing 100190 China"},{"name":"School of Physical Sciences University of Chinese Academy of Sciences  Beijing 100049 China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Xiao","family":"Deng","sequence":"additional","affiliation":[{"name":"Spallation Neutron Source Science Center  Dongguan 523803 China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Jie","family":"Zheng","sequence":"additional","affiliation":[{"name":"Beijing National Laboratory for Condensed Matter Physics and Institute of Physics Chinese Academy of Sciences  Beijing 100190 China"},{"name":"School of Physical Sciences University of Chinese Academy of Sciences  Beijing 100049 China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Wenxiao","family":"Shi","sequence":"additional","affiliation":[{"name":"Beijing National Laboratory for Condensed Matter Physics and Institute of Physics Chinese Academy of Sciences  Beijing 100190 China"},{"name":"School of Physical Sciences University of Chinese Academy of Sciences  Beijing 100049 China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Yunzhong","family":"Chen","sequence":"additional","affiliation":[{"name":"Beijing National Laboratory for Condensed Matter Physics and Institute of Physics Chinese Academy of Sciences  Beijing 100190 China"},{"name":"School of Physical Sciences University of Chinese Academy of Sciences  Beijing 100049 China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Baogen","family":"Shen","sequence":"additional","affiliation":[{"name":"Beijing National Laboratory for Condensed Matter Physics and Institute of Physics Chinese Academy of Sciences  Beijing 100190 China"},{"name":"School of Physical Sciences University of Chinese Academy of Sciences  Beijing 100049 China"},{"name":"Ningbo Institute of Materials Technology &amp; 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