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Starch has been widely used in foods such as noodles, and puddings for thousands of years, but with low mechanical performance. Here, a starch chain phase separation strategy is proposed in synthesizing starch\u2010based hydrogel to simultaneously enhance its strength and toughness, by the tunable interplay of glycerol\/water (as \u2010good solvent) and ethanol (as antisolvent). The mechanical performance of starch hydrogel, composed of starch, bound water, and glycerol, is widely tuned with maximum strains: 194.4\u2013361.4%; maximum tensile stresses: 34\u2013192\u00a0kPa; and Young's moduli: 36.0\u2013205.8\u00a0kPa. Modulating the glycerol\/ethanol ratio governs phase separation dynamics during the structural formation of starch hydrogel: lower glycerol\/ethanol ratios bring higher maximum strain and maximum tensile stress, correlating with reconfigured starch crystallization and dynamic hydrogen\u2010bonding network. Notably, the hyperelastic starch hydrogel achieves complete soil degradation within 24 days and is constructed for a pneumatic soft gripper. This work pioneers a green and sustainable hydrogel platform that harmonizes high performance with edibility and biodegradability, offering transformative potential for eco\u2010friendly soft robotics and transient wearable systems.<\/jats:p>","DOI":"10.1002\/advs.202507216","type":"journal-article","created":{"date-parts":[[2025,7,7]],"date-time":"2025-07-07T03:18:06Z","timestamp":1751858286000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":9,"title":["Hyperelastic Starch Hydrogel Configures Edible and Biodegradable All\u2010Components for Soft Robots"],"prefix":"10.1002","volume":"13","author":[{"given":"Siyu","family":"Yao","sequence":"first","affiliation":[{"name":"College of Biosystems Engineering and Food Science National Engineering Laboratory of Intelligent Food Technology and Equipment Zhejiang Key Laboratory for Agro\u2010Food Processing Fuli Institute of Food Science Zhejiang University  Hangzhou 310058 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Haohao","family":"Hu","sequence":"additional","affiliation":[{"name":"College of Biosystems Engineering and Food Science National Engineering Laboratory of Intelligent Food Technology and Equipment Zhejiang Key Laboratory for Agro\u2010Food Processing Fuli Institute of Food Science Zhejiang University  Hangzhou 310058 China"},{"name":"Innovation Center of Yangtze River Delta Zhejiang University  Jiaxing 314102 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Mengfan","family":"Zhang","sequence":"additional","affiliation":[{"name":"Department of Engineering Mechanics Zhejiang University  Hangzhou 310027 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qingqing","family":"Zhu","sequence":"additional","affiliation":[{"name":"College of Biosystems Engineering and Food Science National Engineering Laboratory of Intelligent Food Technology and Equipment Zhejiang Key Laboratory for Agro\u2010Food Processing Fuli Institute of Food Science Zhejiang University  Hangzhou 310058 China"},{"name":"Innovation Center of Yangtze River Delta Zhejiang University  Jiaxing 314102 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Donghong","family":"Liu","sequence":"additional","affiliation":[{"name":"College of Biosystems Engineering and Food Science National Engineering Laboratory of Intelligent Food Technology and Equipment Zhejiang Key Laboratory for Agro\u2010Food Processing Fuli Institute of Food Science Zhejiang University  Hangzhou 310058 China"},{"name":"Innovation Center of Yangtze River Delta Zhejiang University  Jiaxing 314102 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shaoxing","family":"Qu","sequence":"additional","affiliation":[{"name":"Department of Engineering Mechanics Zhejiang University  Hangzhou 310027 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-7570-6206","authenticated-orcid":false,"given":"Guoyong","family":"Mao","sequence":"additional","affiliation":[{"name":"Department of Engineering Mechanics Zhejiang University  Hangzhou 310027 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Enbo","family":"Xu","sequence":"additional","affiliation":[{"name":"College of Biosystems Engineering and Food Science National Engineering Laboratory of Intelligent Food Technology and Equipment Zhejiang Key Laboratory for Agro\u2010Food Processing Fuli Institute of Food Science Zhejiang University  Hangzhou 310058 China"},{"name":"Innovation Center of Yangtze River Delta Zhejiang University  Jiaxing 314102 China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2025,7,7]]},"reference":[{"key":"e_1_2_9_1_1","doi-asserted-by":"publisher","DOI":"10.1038\/502615a"},{"key":"e_1_2_9_2_1","doi-asserted-by":"publisher","DOI":"10.1039\/C8TB01971A"},{"key":"e_1_2_9_3_1","doi-asserted-by":"publisher","DOI":"10.3389\/fbioe.2020.00461"},{"key":"e_1_2_9_4_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsami.2c22158"},{"key":"e_1_2_9_5_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsami.1c23567"},{"key":"e_1_2_9_6_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.202311214"},{"key":"e_1_2_9_7_1","volume":"8","author":"Xia X.","year":"2024","journal-title":"Macromol. 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