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The core performance of these materials lies in the synergistic optimization of their mechanical properties and interfacial adhesive strength. Although supramolecular hydrogels have achieved initial breakthroughs through dynamic bond design, they fail to be mechanically tough and favorably adhesive underwater at the same time. To address this challenge, a strategy to fabricate a supramolecular hydrogel with high crosslinking density using 3D printing technology is proposed. The obtained hydrogel demonstrates excellent mechanical strength due to its high\u2010density hydrogen bonding crosslinks that it retains a tensile stress of 4\u00a0MPa and can support a 20\u00a0g load without deformation after submersion in water for 30\u00a0min. Meanwhile, it displays remarkable self\u2010adhesion property underwater, achieving an interfacial adhesion strength of 690\u00a0kPa following 20 min of contact duration. Notably, the hydrogel manifests versatile underwater adhesion capabilities to various substrates. Therefore, a supramolecular hydrogel that integrates both good mechanical performance and adhesion underwater characteristics is successfully developed. In addition, modular soft robots are also constructed using this hydrogel, which is able to successfully complete various underwater missions.<\/jats:p>","DOI":"10.1002\/advs.202509542","type":"journal-article","created":{"date-parts":[[2025,9,15]],"date-time":"2025-09-15T19:53:54Z","timestamp":1757966034000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":14,"title":["Supramolecular Hydrogel Showing Mechanical Robustness and Good Adhesion Underwater"],"prefix":"10.1002","volume":"12","author":[{"given":"Xiaohe","family":"Zhou","sequence":"first","affiliation":[{"name":"Department Key Laboratory of Material Chemistry for Energy Conversion and Storage Ministry of Education Hubei Key Laboratory of Material Chemistry and Service Failure Hubei Engineering Research Center for Biomaterials and Medical Protective Materials State Key Laboratory of Materials Processing and Die and Mould Technology School of Chemistry and Chemical Engineering Huazhong University of Science and Technology  Wuhan 430074 P. 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China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Rui","family":"Hu","sequence":"additional","affiliation":[{"name":"Department Key Laboratory of Material Chemistry for Energy Conversion and Storage Ministry of Education Hubei Key Laboratory of Material Chemistry and Service Failure Hubei Engineering Research Center for Biomaterials and Medical Protective Materials State Key Laboratory of Materials Processing and Die and Mould Technology School of Chemistry and Chemical Engineering Huazhong University of Science and Technology  Wuhan 430074 P. R. 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