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Yet its development is hindered by limited strategies to achieve uniform film thickness and homogeneous phase morphology. In this work, an SS process is developed\u00a0using the green solvent o\u2010xylene and mediated by solid additives to regulate interfacial tension, enabling the formation of uniform SS\u2010films on the water surface. The aromatic solid additive phenanthrene (PAT) extended the drying time of the wet film, effectively suppressed excessive acceptor aggregation, enhanced molecular packing order, and optimized phase\u2010separated morphology for the SS\u2010film. The OPV device with SS\u2010film as the active layer achieved a champion efficiency of 16.4%. To the best of current knowledge, this is the first attempt to introduce solid additives in SS\u2010processed OPVs, offering a versatile strategy to simultaneously adjust film\u2010forming kinetics and phase morphology. This study presents a simple approach to fabricating solution OPVs with solution processability and reproducibility.<\/jats:p>","DOI":"10.1002\/advs.202512384","type":"journal-article","created":{"date-parts":[[2025,8,26]],"date-time":"2025-08-26T08:44:30Z","timestamp":1756197870000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":7,"title":["Solid Additives for Spontaneously Spreading\u2010Processed Organic Photovoltaics"],"prefix":"10.1002","volume":"12","author":[{"given":"Huitong","family":"Deng","sequence":"first","affiliation":[{"name":"Zhejiang University  Hangzhou Zhejiang 310027 China"},{"name":"Zhejiang Key Laboratory of 3D Micro\/Nano Fabrication and Characterization Research Center for Industries of the Future Department of Electronic and Information Engineering School of Engineering Westlake University  Hangzhou Zhejiang 310030 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qianqing","family":"Jiang","sequence":"additional","affiliation":[{"name":"Zhejiang Key Laboratory of 3D Micro\/Nano Fabrication and Characterization Research Center for Industries of the Future Department of Electronic and Information Engineering School of Engineering Westlake University  Hangzhou Zhejiang 310030 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-7288-1108","authenticated-orcid":false,"given":"Dianyi","family":"Liu","sequence":"additional","affiliation":[{"name":"Zhejiang University  Hangzhou Zhejiang 310027 China"},{"name":"Zhejiang Key Laboratory of 3D Micro\/Nano Fabrication and Characterization Research Center for Industries of the Future Department of Electronic and Information Engineering School of Engineering Westlake University  Hangzhou Zhejiang 310030 China"},{"name":"Westlake Institute for Optoelectronics  Hangzhou Zhejiang 311421 China"},{"name":"Division of Solar Energy Conversion and Catalysis at Westlake University Zhejiang Baima Lake Laboratory Co., Ltd.  Hangzhou Zhejiang 310000 China"},{"name":"Westlake Optoelectronic Technology Co., Ltd.  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