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Although their molecular structures are similar, significant differences in energy splitting and spin\u2010orbit coupling between the singlet and triplet excited states are exhibited, resulting from the differences in steric configurations and consequent electronic structures. The Th\u2010Cz\u2010BN3 and Th\u2010Cz\u2010BN6\u2010based devices display pure green emission with Commission Internationale de L'Eclairage (CIE) y values exceeding 0.7 and maximum external quantum efficiencies of over 34.0%. Moreover, the Th\u2010Cz\u2010BN3\u2010based non\u2010sensitized device exhibits remarkable efficiency roll\u2010offs of 0.3 and 16.8% at 100 and 1000\u00a0cd m\n                    <jats:sup>\u22122<\/jats:sup>\n                    , respectively, which can be ascribed to the rapid rates of radiative transition and reverse intersystem crossing processes. The results not only achieve sulfur\u2010embedded pure green MR\u2010TADF emitters but also pave the way for designing highly efficient MR\u2010TADF emitters with suppressed efficiency roll\u2010offs.\n                  <\/jats:p>","DOI":"10.1002\/advs.202512796","type":"journal-article","created":{"date-parts":[[2025,10,29]],"date-time":"2025-10-29T20:49:21Z","timestamp":1761770961000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":5,"title":["Sulfur\u2010Embedded Pure Green Multiple Resonance TADF Emitters: Optimizing Photophysical and Electroluminescent Properties"],"prefix":"10.1002","volume":"13","author":[{"given":"Chao","family":"Jiang","sequence":"first","affiliation":[{"name":"Department of Materials Science and Technology Jihua Laboratory 28 Huandao Nan Road Foshan Guangdong Province 528000 P. R. 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