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The conducting polymer poly(3,4\u2010ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS) has emerged as a key bioelectronic material due to its unique properties, processing versatility, and biocompatibility. This work provides an overview of PEDOT:PSS\u2010based bioelectronic interfaces and their growing potential in clinical applications. The historical development of PEDOT:PSS is first traced, highlighting its rise as one of the most successful materials in organic bioelectronics. The fundamental properties that make PEDOT:PSS particularly well\u2010suited for bioelectronic interfaces are then examined, with a focus on how these properties can be precisely tuned through advanced processing and fabrication techniques. Both well\u2010established micropatterned interfaces and the latest advancements in multidimensional hydrogel\u2010based structures are discussed. 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