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However, in these devices, fundamental exploration of ion intercalation\u2010induced structural phase transitions remains largely overlooked and rarely explored. Here, the lithium\u2010based electrolyte gating technique is used to probe the collective interactions between ions, lattices, and electrons in a van der Waals ferroelectric semiconductor \u03b1\u2010In\n                    <jats:sub>2<\/jats:sub>\n                    Se\n                    <jats:sub>3<\/jats:sub>\n                    . Using a polymer electrolyte as the lithium\u2010ion reservoir and \u03b1\u2010In\n                    <jats:sub>2<\/jats:sub>\n                    Se\n                    <jats:sub>3<\/jats:sub>\n                    as the channel material, the intercalated lithium concentration via a gate electric field is modulated. This manipulation drives a phase transition in \u03b1\u2010In\n                    <jats:sub>2<\/jats:sub>\n                    Se\n                    <jats:sub>3<\/jats:sub>\n                    from a ferroelectric semiconductor to a dirty metal and finally to a metal, accompanied by a structural transformation. Concurrently, with enhanced intercalation, the ferroelectric hysteresis window progressively narrows and eventually disappears, indicating the evolution from switchable to non\u2010switchable polarization. This study represents a promising platform for the artificial construction of correlated material systems, enabling a systematic investigation into the interaction of ferroelectricity and electronic conduction using ion intercalation.\n                  <\/jats:p>","DOI":"10.1002\/advs.202513712","type":"journal-article","created":{"date-parts":[[2025,12,13]],"date-time":"2025-12-13T03:37:35Z","timestamp":1765597055000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":2,"title":["Intercalation\u2010Induced Phase Transitions in Ferroelectric \u03b1\u2010In\n                    <sub>2<\/sub>\n                    Se\n                    <sub>3<\/sub>"],"prefix":"10.1002","volume":"13","author":[{"given":"Xin","family":"He","sequence":"first","affiliation":[{"name":"Center for Quantum Matter School of Physics Zhejiang University  Hangzhou 310058 China"},{"name":"ZJU\u2010Hangzhou Global Scientific and Technological Innovation 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