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These\u00a0findings are further correlated with the magnetic properties of the same set of compounds reported in prior studies. The work revealed that the SOX emission intensities and linewidths are mainly controlled by the magnetic anisotropy and spin orientations, and are strongly suppressed by the introduction of substituents. The suppression depends on the type of substituent, with Fe affecting the SOX emission more than Mn and Cr. The 2\u00a0\n                    <jats:sc>m<\/jats:sc>\n                    scattering is linked to short\u2010range correlations and exhibits greater resiliency against metal atom substitution. While the 2M\u00a0 peak at low temperature gets suppressed and red\u2010shifted in frequency with increasing concentrations of all the substituents, Fe induces the weakest suppression compared to all other substituents. Altogether, these findings revealed the introduction of substituents as a powerful route to control the emergent collective excitations in NiPS\n                    <jats:sub>3<\/jats:sub>\n                    and mixed\u2010MPX\n                    <jats:sub>3<\/jats:sub>\n                    materials.\n                  <\/jats:p>","DOI":"10.1002\/advs.202517378","type":"journal-article","created":{"date-parts":[[2025,12,13]],"date-time":"2025-12-13T01:54:15Z","timestamp":1765590855000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Manipulation of Emergent Collective Excitations via Composition Control in Mixed MPX\n                    <sub>3<\/sub>\n                    Correlated 2D Antiferromagnets"],"prefix":"10.1002","volume":"13","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-1642-4313","authenticated-orcid":false,"given":"Cong Tai","family":"Trinh","sequence":"first","affiliation":[{"name":"Center for Integrated Nanotechnologies Materials Physics and Applications Division Los Alamos National Laboratory  Los Alamos NM 87545 USA"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0009-0000-1220-7525","authenticated-orcid":false,"given":"Na","family":"Liu","sequence":"additional","affiliation":[{"name":"Center for Integrated Nanotechnologies Materials Physics and Applications Division Los Alamos National Laboratory  Los Alamos NM 87545 USA"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-5511-3155","authenticated-orcid":false,"given":"Rabindra","family":"Basnet","sequence":"additional","affiliation":[{"name":"Department of Physics University of Arkansas  Fayetteville AR 72701 USA"},{"name":"Department of Physics Morgan State University  Baltimore MD 21251 USA"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0009-0008-3161-3156","authenticated-orcid":false,"given":"Dinesh","family":"Upreti","sequence":"additional","affiliation":[{"name":"Department of Physics University of Arkansas  Fayetteville AR 72701 USA"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-0124-5213","authenticated-orcid":false,"given":"Rijan","family":"Karkee","sequence":"additional","affiliation":[{"name":"Center for Integrated Nanotechnologies Materials Physics and Applications Division Los Alamos National Laboratory  Los Alamos NM 87545 USA"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-6014-9953","authenticated-orcid":false,"given":"Vigneshwaran","family":"Chandrasekaran","sequence":"additional","affiliation":[{"name":"Center for Integrated Nanotechnologies Materials Physics and Applications Division Los Alamos National Laboratory  Los Alamos NM 87545 USA"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-9205-4847","authenticated-orcid":false,"given":"Andrew C.","family":"Jones","sequence":"additional","affiliation":[{"name":"Center for Integrated Nanotechnologies Materials Physics and Applications Division Los Alamos National Laboratory  Los Alamos NM 87545 USA"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-6862-6841","authenticated-orcid":false,"given":"Michael T.","family":"Pettes","sequence":"additional","affiliation":[{"name":"Center for Integrated Nanotechnologies Materials Physics and Applications Division Los Alamos National Laboratory  Los Alamos NM 87545 USA"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-0062-8821","authenticated-orcid":false,"given":"Thuc T.","family":"Mai","sequence":"additional","affiliation":[{"name":"Materials and Manufacturing Directorate Air Force Research Laboratory  Wright\u2010Patterson Air Force Base OH 45433 USA"},{"name":"BlueHalo Inc.  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