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However, lithium\u2010excess high\u2010temperature synthesis generates substantial residual lithium compounds (RLCs; e.g., Li\n                    <jats:sub>2<\/jats:sub>\n                    CO\n                    <jats:sub>3<\/jats:sub>\n                    \/LiOH) on particle surfaces. These RLCs elevate interfacial impedance, while protracted Li\u207a diffusion pathways in micrometer\u2010sized crystals collectively degrade fast\u2010charge capability and cycling stability. To address these challenges, we develop an efficient strategy employing 3\u2010min ultrafast washing followed by 600\u00b0C annealing for LiNi\n                    <jats:sub>0.85<\/jats:sub>\n                    Co\n                    <jats:sub>0.1<\/jats:sub>\n                    Mn\n                    <jats:sub>0.05<\/jats:sub>\n                    O\n                    <jats:sub>2<\/jats:sub>\n                    single crystals. This approach achieves 80% capacity retention at 5 C charging meeting extreme fast\u2010charging targets while maintaining superior cycling stability at 1 C. The ultrafast wash removes 94.5% of surface RLCs while confining structural deterioration to a mere 2\u20134\u00a0nm rock\u2010salt reconstruction layer. Complementarily, in situ X\u2010ray diffraction (XRD) reveals that this attenuated surface rock\u2010salt phase enables smooth bulk phase transitions during Li\n                    <jats:sup>+<\/jats:sup>\n                    (de)intercalation, thereby enhancing structural reversibility, ionic conductivity, and long\u2010term stability.\n                  <\/jats:p>","DOI":"10.1002\/advs.202517421","type":"journal-article","created":{"date-parts":[[2025,12,24]],"date-time":"2025-12-24T03:46:42Z","timestamp":1766548002000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":7,"title":["Achieving Fast Charging and Superior Cycling Stability Single\u2010Crystal Ni\u2010Rich Cathodes by Ultrafast Aqueous Washing"],"prefix":"10.1002","volume":"13","author":[{"given":"Kaixin","family":"Liu","sequence":"first","affiliation":[{"name":"School of Materials and New Energy Ningxia University  Yinchuan China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jia","family":"Yang","sequence":"additional","affiliation":[{"name":"School of Materials and New Energy Ningxia University  Yinchuan China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Huaping","family":"Wang","sequence":"additional","affiliation":[{"name":"School of Materials and New Energy Ningxia University  Yinchuan China"},{"name":"Helanshan Laboratory  Yinchuan China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yongtao","family":"Tan","sequence":"additional","affiliation":[{"name":"School of Materials and New Energy Ningxia University  Yinchuan China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Dongdong","family":"Fan","sequence":"additional","affiliation":[{"name":"School of Materials and New Energy Ningxia University  Yinchuan China"},{"name":"Helanshan Laboratory  Yinchuan China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yongjian","family":"Cui","sequence":"additional","affiliation":[{"name":"School of Materials and New Energy Ningxia University  Yinchuan China"},{"name":"Helanshan Laboratory  Yinchuan China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"YunJian","family":"Liu","sequence":"additional","affiliation":[{"name":"School of Materials Science &amp; Engineering Jiangsu University  Zhenjiang China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiaoyan","family":"Li","sequence":"additional","affiliation":[{"name":"Ningxia Hanyao Rich Lithium Technology Co., Ltd.  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