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Interfacial dislocations, such as stacking faults (SF) and rotational misorientations (RM), are typically unavoidable and play a key role in shaping their interlayer transport properties. However, the absence of techniques to decouple their individual contributions has hindered a quantitative understanding of how stacking states affect interlayer electrical transport, even in well\u2010studied materials like graphite. In this work, we measure the intrinsic c\u2010axis resistivity of AB\u2010stacked epitaxial single\u2010crystal graphite (5.7 \u00d7 10\n                    <jats:sup>\u22125<\/jats:sup>\n                    \u2005\u03a9 \u00b7 m) through high\u2010throughput measurements at room temperature. We further develop a decoupling strategy that combines rotational locking of highly oriented pyrolytic graphite (HOPG) with in situ measurements. Comparative analysis enable us to quantify, for the first time, the interlayer effective resistivity ratio of RM:SF:AB stacking as approximately 4507:74:1. In addition, we extend our methodology by introducing a large\u2010scale, pixel\u2010array\u2010based lateral measurement technique that reveals the internal dislocation structures and their tunability in vdW materials from a new spatial perspective. This work marks a significant advance in elucidating graphite's c\u2010axis electrical transport, providing a robust framework for investigating vdW materials with complex stacking structures.\n                  <\/jats:p>","DOI":"10.1002\/advs.202518254","type":"journal-article","created":{"date-parts":[[2026,1,7]],"date-time":"2026-01-07T15:35:09Z","timestamp":1767800109000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":2,"title":["Origins of Graphite Resistivity: Decoupling Stacking Fault and Rotational Misorientation"],"prefix":"10.1002","volume":"13","author":[{"ORCID":"https:\/\/orcid.org\/0009-0004-5175-6868","authenticated-orcid":false,"given":"Weipeng","family":"Chen","sequence":"first","affiliation":[{"name":"College of Mechatronics and Control Engineering Shenzhen University  Shenzhen China"},{"name":"Center for Nano and Micro Mechanics Tsinghua University  Beijing China"},{"name":"Department of Engineering Mechanics School of Aerospace Engineering Tsinghua University  Beijing China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Fuwei","family":"Yang","sequence":"additional","affiliation":[{"name":"Center for Nano and Micro Mechanics Tsinghua University  Beijing China"},{"name":"Department of Engineering Mechanics School of Aerospace Engineering Tsinghua University  Beijing China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Tielin","family":"Wu","sequence":"additional","affiliation":[{"name":"Center for Nano and Micro Mechanics Tsinghua University  Beijing China"},{"name":"Department of Engineering Mechanics School of Aerospace Engineering Tsinghua University  Beijing China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yelingyi","family":"Wang","sequence":"additional","affiliation":[{"name":"Center for Nano and Micro Mechanics Tsinghua University  Beijing China"},{"name":"Department of Engineering Mechanics School of Aerospace Engineering Tsinghua University  Beijing China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Quanshui","family":"Zheng","sequence":"additional","affiliation":[{"name":"Center for Nano and Micro Mechanics Tsinghua University  Beijing China"},{"name":"Department of Engineering Mechanics School of Aerospace Engineering Tsinghua University  Beijing China"},{"name":"Institute of Superlubricity Technology Research Institute of Tsinghua University in Shenzhen  Shenzhen China"},{"name":"Tsinghua Shenzhen International Graduate School  Shenzhen China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Deli","family":"Peng","sequence":"additional","affiliation":[{"name":"Tsinghua Shenzhen International Graduate School  Shenzhen China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-2505-0050","authenticated-orcid":false,"given":"Zhanghui","family":"Wu","sequence":"additional","affiliation":[{"name":"College of 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