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However, the roles of microstructure and viscoelasticity on EDL\u2010driven sensing remain poorly understood. This study establishes detailed correlations between elastomer microstructure, intrinsic viscoelastic properties, and sensor performance by integrating mechanical and electrical analyses. Validation of the EDL mechanism reveals how microstructural optimization and viscoelastic tuning enhance sensitivity, linear range, and stability. Height\u2010graded architectures yield a sensor with a sensitivity of 2.70\u00a0nF\/kPa, a broad linear range of 0\u20132000\u00a0kPa, and robust durability over 10\u00a0000 cycles. These devices demonstrate multifunctionality in robotic electronic skin, pressure mapping, and real\u2010time physiological monitoring such as wrist pulse detection. The findings establish key structure\u2013property\u2013performance relationships, providing design guidelines for next\u2010generation, high\u2010performance super\u2010capacitive sensors.<\/jats:p>","DOI":"10.1002\/advs.202519398","type":"journal-article","created":{"date-parts":[[2026,1,22]],"date-time":"2026-01-22T16:40:26Z","timestamp":1769100026000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":4,"title":["Understanding the Roles of Microstructure and Viscoelasticity of Soft Ionic Elastomer for Super\u2010Capacitive Pressure Sensors"],"prefix":"10.1002","volume":"13","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-1895-0405","authenticated-orcid":false,"given":"Allen J.","family":"Cheng","sequence":"first","affiliation":[{"name":"School of Mechanical and Manufacturing Engineering University of New South Wales  Sydney New South Wales 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