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In this report, we propose a universal interfacing design strategy for the fabrication of versatile conductive MXene coatings on the surface of flexible organic crystals that preserve the electric conductivity of the MXenes while they also remain mechanically flexible and robust across a wide temperature range of nearly 300\u00b0C both above and below ambient temperature. This new sub\u2010class of hybrid materials based on adaptive organic crystals undergoes reversible changes in the crystal structure upon deformation, while they also engender stable electrical conductivity and retain deformation sensitivity from about \u2212196\u00b0C to 100\u00b0C. A wireless sensing system based on these materials was constructed to monitor bionic finger movements that demonstrate the potential for human\u2010machine interfacing and medical monitoring applications. The structural stability of this and similar devices that utilize crystal\u2010MXene hybrid materials under non\u2010ambient temperatures provide an innovative solution to the current challenges with occasional failure of low\u2010temperature mechanical sensing systems in extreme environments, and specifically such that are used in lunar and deep\u2010space explorations.<\/jats:p>","DOI":"10.1002\/advs.202522007","type":"journal-article","created":{"date-parts":[[2026,3,30]],"date-time":"2026-03-30T19:18:43Z","timestamp":1774898323000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":3,"title":["Organic Crystal\u2010MXene Composites as Temperature\u2010Tolerant Strain Sensors"],"prefix":"10.1002","volume":"13","author":[{"given":"Xuesong","family":"Yang","sequence":"first","affiliation":[{"name":"State Key Laboratory of Supramolecular Structure and Materials College of Chemistry Jilin University  Changchun P. R. 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