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Conventional van der Waals coatings yield unstable interfaces and poor ion\/electron transport, while thermal transport remains underexplored. Here, we propose heterointerface\u2010engineered Si@MoSe\n                    <jats:sub>2<\/jats:sub>\n                    @C anodes with chemically bonded interfaces, where lattice\u2010matched MoSe\n                    <jats:sub>2<\/jats:sub>\n                    covalently bridges porous Si and carbon coating, forming robust Si\u2500Se\u2500Mo linkages that stabilize the structure and optimize transport pathways. The Si@MoSe\n                    <jats:sub>2<\/jats:sub>\n                    @C anode delivers 1054\u00a0mAh g\n                    <jats:sup>\u22121<\/jats:sup>\n                    after 100 cycles at 0.2 A g\n                    <jats:sup>\u22121<\/jats:sup>\n                    \u2014exceeding most Si anodes\u2014and 99.5% Coulombic efficiency over 400 cycles at 1.0 A g\n                    <jats:sup>\u22121<\/jats:sup>\n                    , with high cycling efficiency demonstrated in both liquid and all\u2010solid\u2010state lithium\u2010ion batteries (ASSLIBs). In situ X\u2010ray diffraction, Raman spectroscopy, and electron microscopy\/spectroscopy, together with first\u2010principles calculations, confirm that this MoSe\n                    <jats:sub>2<\/jats:sub>\n                    \u2010mediated covalent bridging enables reversible reactions with favorable kinetics and structural integrity by strengthening and delocalizing Se\u2500Si bonding and reducing Li\n                    <jats:sup>+<\/jats:sup>\n                    migration barriers by 24%. Critically, we present the first measurements of the effective thermal conductivity of a silicon\u2010anode composite, showing that Si@MoSe\n                    <jats:sub>2<\/jats:sub>\n                    @C exhibits a 27% higher value than Si, addressing long\u2010overlooked cell\u2010level thermal\u2010management requirements and improving elevated\u2010temperature cell performance. This heterointerface design provides a synergistic strategy for engineering high\u2010performance Si anodes across batteries with enhanced safety.\n                  <\/jats:p>","DOI":"10.1002\/advs.202523320","type":"journal-article","created":{"date-parts":[[2026,1,31]],"date-time":"2026-01-31T19:48:01Z","timestamp":1769888881000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":5,"title":["A Si\u2010MoSe\n                    <sub>2<\/sub>\n                    Heterostructured Anode with Enhanced Thermal Transport and Electrochemical Performance for Liquid and All\u2010Solid\u2010State Lithium\u2010Ion Batteries"],"prefix":"10.1002","volume":"13","author":[{"given":"Yajun","family":"Zhu","sequence":"first","affiliation":[{"name":"Key Laboratory of Functional Molecular Solids Ministry of Education College of Chemistry and Materials Science Anhui Normal University  Wuhu Anhui P. R. 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