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Here, an electrochemical model based on multi\u2010scale microstructural images was established to identify lithium plating\u2010stripping processes, thereby supporting the predictive outcomes of electrochemical monitoring techniques. Experiments revealed that the open\u2010circuit voltage differential curve (dOCV\/dt) led to ambiguous delineation of the safe state\u2010of\u2010charge (SOC) operating range. The established lithium plating\u2010stripping model was used to compare with experimental results, revealing the dynamic evolution of electrode\u2010scale kinetics and quantified the impact of lithium metal residue on electrode performance. Ex situ X\u2010ray computed tomography (XCT) captured micrometer\u2010resolution microstructural details of graphite electrodes and plated lithium, enabling further correlation of spatially heterogeneous lithium plating\u2010stripping reactions with electrode microstructure. The sensitivity of lithium plating to electrode microstructure was examined at the particle scale, attributed to competition between electrode kinetic rates and active reaction areas. Theoretical mechanism analysis and experimental results from high\u2010energy\u2010density electrodes demonstrated that positioning small particles on the current collector side effectively mitigates solid\u2010state diffusion polarization while confining side reactions to a limited area. The integration of experiments and multiscale modeling elucidates the relationship between lithium plating\u2010stripping reactions and electrode structure, providing mechanistic insights for similar structural optimization designs.<\/jats:p>","DOI":"10.1002\/advs.202524109","type":"journal-article","created":{"date-parts":[[2026,3,25]],"date-time":"2026-03-25T19:29:38Z","timestamp":1774466978000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":2,"title":["Microstructure\u2010Resolved Modeling to Predicting and Regulating Lithium Plating\u2010Stripping Dynamics on Graphite Electrodes"],"prefix":"10.1002","volume":"13","author":[{"given":"Heng","family":"Huang","sequence":"first","affiliation":[{"name":"Key Laboratory of Ocean Energy Utilization and Energy Conservation of Ministry of Education Dalian University of Technology  Dalian 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