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Here, we overturn this paradigm by demonstrating that sub\u2010\n                    <jats:italic>T<\/jats:italic>\n                    <jats:sub>g<\/jats:sub>\n                    annealing simultaneously increases both the strength and compressive plasticity of a chemically tailored Zr\u2010based metallic glass, with plastic strain increasing by &gt;150%. Our experimental analyses reveal that strategically employed Ni\u2500Cu repulsion drives elemental partitioning during annealing, which seeds nanoscale chemical heterogeneity. Concurrently, atomistic simulations suggest the emergence of locally densely\u2010packed regions (LDPRs) with characteristically low activation energy for shear transformation. These findings indicate that plasticity can be sustained by heterogeneous structures wherein densely\u2010packed motifs, alongside conventional loosely\u2010packed regions, serve as potential shear transformation sites. This shifts the design paradigm from merely introducing LLPRs to strategically engineering heterogeneous structures that enable compensatory plasticity.\n                  <\/jats:p>","DOI":"10.1002\/advs.202524294","type":"journal-article","created":{"date-parts":[[2026,3,8]],"date-time":"2026-03-08T21:24:50Z","timestamp":1773005090000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Annealing\u2010Induced Plasticity and Strengthening in Metallic Glasses"],"prefix":"10.1002","volume":"13","author":[{"ORCID":"https:\/\/orcid.org\/0000-0001-9264-9963","authenticated-orcid":false,"given":"Yingjie","family":"Zhang","sequence":"first","affiliation":[{"name":"State Key Laboratory for Advanced Metals and Materials University of Science and Technology Beijing  Beijing China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jinyue","family":"Wang","sequence":"additional","affiliation":[{"name":"State Key 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