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While bioplastics hold promise as alternatives, their limited heat resistance and shaping capabilities hinder widespread adoption in high\u2010performance engineering. Here, we present an innovative supramolecular network that utilizes cellulose as a molecular framework, complemented by acrylamide molecules for in situ polymerization. By applying ethanol for structural reconstruction, we create a self\u2010reinforcing bioplastic (S\u2010bioplastic) with a tensile strength of 76\u00a0MPa and a flexural modulus of 4.7\u00a0GPa. This S\u2010bioplastic supports multiple molding techniques\u2014such as injection and compression molding\u2014and exhibits remarkable environmental adaptability, with thermal stability up to 180\u00b0C and low\u2010temperature resilience to \u2212196\u00b0C. Compared to conventional plastics, S\u2010bioplastic offers enhanced mechanical properties, biocompatibility, biodegradability, and recyclability, achieving a 95% retention of strength. A techno\u2010economic analysis underscores its value proposition. This research highlights a method for converting bamboo\u2010based materials into high\u2010value bioplastics, providing a promising strategy to address plastic pollution while developing lightweight, high\u2010performance materials for aerospace applications.<\/jats:p>","DOI":"10.1002\/advs.74426","type":"journal-article","created":{"date-parts":[[2026,2,15]],"date-time":"2026-02-15T11:53:15Z","timestamp":1771156395000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":12,"title":["Stimulus\u2010Induced Self\u2010Reinforcement in Supramolecular Bamboo Plastics toward Mechanical Robustness and Programmable Shapeability"],"prefix":"10.1002","volume":"13","author":[{"given":"Jingcai","family":"Li","sequence":"first","affiliation":[{"name":"Key Laboratory On Resources Chemicals and Materials of Ministry of Education Shenyang University of Chemical Technology  Shenyang P. R. 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