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With only 0.15 wt.% Pd, the hydrothermally treated catalyst (Pd\/SnO\n                    <jats:sub>2<\/jats:sub>\n                    \u2010H) exhibits a reaction rate three times that of the fresh counterpart (Pd\/SnO\n                    <jats:sub>2<\/jats:sub>\n                    \u2010F). Combined experimental and theoretical evidence reveals that hydrothermal treatment redistributes Pd species and partially incorporates Pd atoms into the SnO\n                    <jats:sub>2<\/jats:sub>\n                    lattice, generating single\u2010atom Pd sites (Pd\n                    <jats:sub>1<\/jats:sub>\n                    ). These lattice\u2010incorporated Pd\n                    <jats:sub>1<\/jats:sub>\n                    sites strengthen the Pd\u2010SnO\n                    <jats:sub>2<\/jats:sub>\n                    interaction, which weakens the Pd\u2500O bond, thereby promoting the formation of oxygen vacancies and, more importantly, facilitating the subsequent rate\u2010determining O\n                    <jats:sub>2<\/jats:sub>\n                    activation step. This enables a low\u2010barrier Mars\u2013van Krevelen pathway, in contrast to the higher\u2010energy Langmuir\u2013Hinshelwood route operating on PdO clusters in Pd\/SnO\n                    <jats:sub>2<\/jats:sub>\n                    \u2010F, thereby explaining the high intrinsic activity of Pd\/SnO\n                    <jats:sub>2<\/jats:sub>\n                    \u2010H. Furthermore, Pd lattice doping modulates the\n                    <jats:italic>d<\/jats:italic>\n                    \u2010electron distribution of Pd and weakens CO adsorption, effectively alleviating the CO poisoning typically observed on conventional Pd nanoparticles. Together, these results establish a new design principle for high\u2010performance single\u2010atom catalysts, demonstrating that lattice\u2011embedding of the active metal into a reducible oxide support can simultaneously enhance redox kinetics and suppress poisoning.\n                  <\/jats:p>","DOI":"10.1002\/advs.75534","type":"journal-article","created":{"date-parts":[[2026,5,5]],"date-time":"2026-05-05T19:52:57Z","timestamp":1778010777000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Hydrothermal Embedding of Pd Single Atoms Into SnO\n                    <sub>2<\/sub>\n                    for Efficient CO Oxidation"],"prefix":"10.1002","volume":"13","author":[{"given":"Yingsheng","family":"An","sequence":"first","affiliation":[{"name":"Laboratory of Atmospheric Environment and Pollution Control Research Center for Eco\u2010Environmental Sciences Chinese Academy of Sciences  Beijing 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