{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,5]],"date-time":"2026-10-05T11:00:16Z","timestamp":1791198016137,"version":"4.1.0"},"reference-count":48,"publisher":"Wiley","issue":"55","license":[{"start":{"date-parts":[[2026,7,11]],"date-time":"2026-07-11T00:00:00Z","timestamp":1783728000000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/creativecommons.org\/licenses\/by\/4.0\/"},{"start":{"date-parts":[[2026,7,11]],"date-time":"2026-07-11T00:00:00Z","timestamp":1783728000000},"content-version":"tdm","delay-in-days":0,"URL":"http:\/\/doi.wiley.com\/10.1002\/tdm_license_1.1"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["22222902"],"award-info":[{"award-number":["22222902"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["advanced.onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["Advanced Science"],"published-print":{"date-parts":[[2026,10]]},"abstract":"<jats:title>ABSTRACT<\/jats:title>\n                  <jats:p>\n                    Aqueous zinc\u2010ion batteries exhibit considerable potential for use in grid\u2010scale energy storage. However, issues such as zinc dendrite growth and the occurrence of the hydrogen evolution reaction have limited their development. To address these challenges, this study develop Ormosil, a water\u2010soluble organosilane additive for the electrolyte. In the electrolyte, Ormosil forms Si\u2500O\u2500Zn bonds with the zinc foil, thereby helping to protect the electrode from corrosion reactions. Moreover, on the electrode surface, it facilitates the formation of a solid\u2010electrolyte\u2010interphase layer, enabling rapid zinc\u2010ion transport kinetics. Notably, the hydrophilicity of the organosilane is enhanced by the introduction of \u2500NH\n                    <jats:sub>2<\/jats:sub>\n                    groups. Furthermore, the \u2500NH\n                    <jats:sub>2<\/jats:sub>\n                    groups can bind to zinc ions and become part of their solvation shell; this incorporation helps suppress the hydrogen evolution reaction. Consequently, the single additive Ormosil provides both electrode protection and solvent restructuring. The cell using Ormosil additive exhibited excellent cycling stability (10\u00a0mA\u00a0cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    , 1000\u00a0h), a high average coulombic efficiency (CE = 99.74%), and a full cell with NVO cathode demonstrated high capacity retention (76.60%), superior to ZnSO\n                    <jats:sub>4<\/jats:sub>\n                    (51.08%).\n                  <\/jats:p>","DOI":"10.1002\/advs.76526","type":"journal-article","created":{"date-parts":[[2026,7,11]],"date-time":"2026-07-11T18:31:51Z","timestamp":1783794711000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":1,"title":["A Bifunctional Organosilane Additive for Dynamic pH Regulation and Interfacial Protection in Aqueous Zinc\u2010Ion Batteries"],"prefix":"10.1002","volume":"13","author":[{"given":"Lina","family":"Pan","sequence":"first","affiliation":[{"name":"School of Chemistry and Materials Science Jiangsu Normal University  Xuzhou P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Haiyang","family":"Wu","sequence":"additional","affiliation":[{"name":"School of Chemistry and Materials Science Jiangsu Normal University  Xuzhou P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Peng","family":"Huang","sequence":"additional","affiliation":[{"name":"School of Chemistry and Materials Science Jiangsu Normal University  Xuzhou P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Boyu","family":"Yuan","sequence":"additional","affiliation":[{"name":"School of Physics and Electronic Engineering Jiangsu Normal University  Xuzhou P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-6021-6343","authenticated-orcid":false,"given":"Chao","family":"Lai","sequence":"additional","affiliation":[{"name":"School of Chemistry and Materials Science Jiangsu Normal University  Xuzhou P. R. 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