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However, natural mechanical energies are typically weak and low\u2010frequency, necessitating materials with high flexibility, facile deformation, and large surface area. Herein, we demonstrate that the ABCABC stacking sequence along the\n                    <jats:italic>c<\/jats:italic>\n                    \u2010axis in two\u2010dimensional (2D) 3R\u2010 zinc indium sulfide (3R\u2010ZnIn\n                    <jats:sub>2<\/jats:sub>\n                    S\n                    <jats:sub>4<\/jats:sub>\n                    ) nanosheets induces intrinsic non\u2010centrosymmetry, enabling robust piezocatalysis for on\u2010site hydrogen peroxide (H\n                    <jats:sub>2<\/jats:sub>\n                    O\n                    <jats:sub>2<\/jats:sub>\n                    ) generation and simultaneous uranium extraction. Density functional theory (DFT) calculations confirm that solvation effects enhance the lattice flexibility and intrinsic dipole moment of 3R\u2010 ZnIn\n                    <jats:sub>2<\/jats:sub>\n                    S\n                    <jats:sub>4<\/jats:sub>\n                    , resulting in the formation of an electron\u2010rich surface that thermodynamically favors the two\u2010electron oxygen reduction reaction (2e\u2212 ORR) for H\n                    <jats:sub>2<\/jats:sub>\n                    O\n                    <jats:sub>2<\/jats:sub>\n                    generation. Under mild ultrasonic agitation (35\u00a0kHz, 50\u00a0W), the 3R\u2010ZnIn\n                    <jats:sub>2<\/jats:sub>\n                    S\n                    <jats:sub>4<\/jats:sub>\n                    nanosheets achieved a H\n                    <jats:sub>2<\/jats:sub>\n                    O\n                    <jats:sub>2<\/jats:sub>\n                    yield of 276.7\u00a0\u00b5mol\u00a0g\n                    <jats:sup>\u22121<\/jats:sup>\n                    \u00a0h\n                    <jats:sup>\u22121<\/jats:sup>\n                    and a uranium extraction capacity of 763.2\u00a0mg\u00a0g\n                    <jats:sup>\u22121<\/jats:sup>\n                    . Mechanistic investigations elucidate that the uranium extraction process proceeds through a dual\u2010coordination pathway, integrating direct piezoelectric reduction and in situ H\n                    <jats:sub>2<\/jats:sub>\n                    O\n                    <jats:sub>2<\/jats:sub>\n                    \u2010mediated complexation of uranium species. Notably, 3R\u2010ZnIn\n                    <jats:sub>2<\/jats:sub>\n                    S\n                    <jats:sub>4<\/jats:sub>\n                    demonstrates excellent cycling stability over five cycles, high selectivity toward uranium, and effective anti\u2010biofouling performance under ultrasonic conditions (35\u00a0kHz, 50\u00a0W). Collectively, our findings establish stacking\u2010induced piezoelectricity as a light\u2010independent strategy for sustainable uranium extraction to support nuclear energy development.\n                  <\/jats:p>","DOI":"10.1002\/advs.76617","type":"journal-article","created":{"date-parts":[[2026,7,16]],"date-time":"2026-07-16T10:17:18Z","timestamp":1784197038000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":1,"title":["ABCABC Stacking\u2010Enabled Non\u2010Centrosymmetry 3R\u2010ZnIn\n                    <sub>2<\/sub>\n                    S\n                    <sub>4<\/sub>\n                    Nanosheets for Piezocatalytic Uranium Extraction"],"prefix":"10.1002","volume":"13","author":[{"given":"Song","family":"Li","sequence":"first","affiliation":[{"name":"School of Materials Science and Engineering School of Interdisciplinary Science Beijing Institute of Technology  Beijing 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