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Here, we develop a coaxial wet\u2010spinning strategy that enables the continuous aqueous\u2010bath confinement of an uncured PDMS\/CNT conductive core. During spinning, a rapidly phase\u2010separating PVDF\u2010HFP sheath provides immediate radial confinement, preventing leakage and structural collapse of the hydrophobic liquid core, while a UV\u2010crosslinked PEGDA secondary network reinforces the sheath after fiber formation. Unlike removable templates or sacrificial supporting layers, the PVDF\u2010HFP\/PEGDA sheath is permanently retained as the dielectric and load\u2010bearing component, thereby directly forming an integrated dielectric\u2013electrode coaxial fiber. The resulting PVDF\u2010HFP\/PEGDA@PDMS\/CNT fibers can be continuously fabricated at the meter scale and exhibit reversible sheath microstructural evolution, stable strain\u2010dependent resistance, and reliable performance under repeated deformation. The integrated dielectric\u2013electrode architecture also allows an individual fiber to generate triboelectric signals without additional device assembly. This work demonstrates a practical route for continuously processing uncured PDMS\u2010based conductive materials in an aqueous coagulation bath and integrating mechanical, resistive, and triboelectric functions within a permanently retained coaxial fiber architecture.<\/jats:p>","DOI":"10.1002\/advs.77580","type":"journal-article","created":{"date-parts":[[2026,9,7]],"date-time":"2026-09-07T04:51:36Z","timestamp":1788756696000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Mechanically Reprogrammed Coaxial Fibers for Multiphysics Transduction and Human\u2010Machine Interfaces"],"prefix":"10.1002","author":[{"given":"Xinyi","family":"Cao","sequence":"first","affiliation":[{"name":"School of Mechanical and Manufacturing Engineering University of New South Wales  Sydney NSW Australia"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-3794-5756","authenticated-orcid":false,"given":"Chao","family":"Ye","sequence":"additional","affiliation":[{"name":"School of Textile and Clothing Yancheng Institute of Technology  Yancheng Jiangsu China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-1156-0479","authenticated-orcid":false,"given":"Shengjie","family":"Ling","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Molecular Engineering of Polymers Department of Macromolecular Science Fudan University  Shanghai China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-7450-6205","authenticated-orcid":false,"given":"Ming","family":"Li","sequence":"additional","affiliation":[{"name":"School of Mechanical and Manufacturing Engineering University of New South Wales  Sydney NSW Australia"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhao","family":"Sha","sequence":"additional","affiliation":[{"name":"Centre for Advanced Manufacturing Technology School of Engineering Faculty of Engineering Computing and Science Western Sydney University  Penrith NSW Australia"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-6081-1487","authenticated-orcid":false,"given":"Chun\u2010Hui","family":"Wang","sequence":"additional","affiliation":[{"name":"School of Mechanical and Manufacturing Engineering University of New South Wales  Sydney NSW Australia"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-5680-9448","authenticated-orcid":false,"given":"Shuhua","family":"Peng","sequence":"additional","affiliation":[{"name":"School of Mechanical and Manufacturing Engineering University of New South Wales  Sydney NSW Australia"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2026,9,6]]},"reference":[{"key":"e_1_2_9_2_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41928\u2010022\u201000723\u2010z"},{"key":"e_1_2_9_3_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467\u2010023\u201042838\u20107"},{"key":"e_1_2_9_4_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.202402815"},{"key":"e_1_2_9_5_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jmst.2024.12.096"},{"key":"e_1_2_9_6_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.73094"},{"key":"e_1_2_9_7_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202203905"},{"key":"e_1_2_9_8_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.202404195"},{"key":"e_1_2_9_9_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202305583"},{"key":"e_1_2_9_10_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41598\u2010019\u201053215\u20100"},{"key":"e_1_2_9_11_1","doi-asserted-by":"crossref","unstructured":"D.Yang A.Fadeev P. N.Adams andB. R.Mattes \u201cControlling Macrovoid Formation in Wet\u2010Spun Polyaniline Fibers \u201dInSmart Structures and Materials 2001: Electroactive Polymer Actuators and Devices(SPIE 2001):59\u201371.","DOI":"10.1117\/12.432691"},{"key":"e_1_2_9_12_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.nanoen.2025.111211"},{"key":"e_1_2_9_13_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41598\u2010017\u201018209\u2010w"},{"key":"e_1_2_9_14_1","doi-asserted-by":"publisher","DOI":"10.1126\/science.ade7341"},{"key":"e_1_2_9_15_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsapm.3c02614"},{"key":"e_1_2_9_16_1","doi-asserted-by":"crossref","first-page":"3519","DOI":"10.1007\/s10570-026-06984-7","article-title":"Dry\u2010Jet Wet\u2010Spun Cellulose Fibers: Coagulation Bath Effects and Straw Cellulose Utilization","volume":"33","author":"Wang C.","year":"2026","journal-title":"Cellulose"},{"key":"e_1_2_9_17_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.nanolett.4c01512"},{"key":"e_1_2_9_18_1","doi-asserted-by":"publisher","DOI":"10.1177\/16878132221095918"},{"key":"e_1_2_9_19_1","doi-asserted-by":"publisher","DOI":"10.1039\/C9NH00519F"},{"key":"e_1_2_9_20_1","doi-asserted-by":"publisher","DOI":"10.1126\/sciadv.adj5407"},{"key":"e_1_2_9_21_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467\u2010021\u201027066\u20101"},{"key":"e_1_2_9_22_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsami.0c08114"},{"key":"e_1_2_9_23_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.sna.2018.10.012"},{"key":"e_1_2_9_24_1","doi-asserted-by":"publisher","DOI":"10.3390\/polym11091433"},{"key":"e_1_2_9_25_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41427\u2010022\u201000359\u20107"},{"key":"e_1_2_9_26_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsaelm.2c01728"},{"key":"e_1_2_9_27_1","doi-asserted-by":"publisher","DOI":"10.3390\/s20236910"},{"key":"e_1_2_9_28_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467\u2010024\u201054442\u20104"},{"key":"e_1_2_9_29_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.nanoen.2023.108823"},{"key":"e_1_2_9_30_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.mtphys.2023.101100"},{"key":"e_1_2_9_31_1","doi-asserted-by":"publisher","DOI":"10.1126\/sciadv.abg4041"},{"key":"e_1_2_9_32_1","doi-asserted-by":"publisher","DOI":"10.1007\/s42765\u2010025\u201000567\u20100"},{"key":"e_1_2_9_33_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.chemrev.3c00196"},{"key":"e_1_2_9_34_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cej.2026.176211"},{"key":"e_1_2_9_35_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.75354"},{"key":"e_1_2_9_36_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.202304809"},{"key":"e_1_2_9_37_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202300447"},{"key":"e_1_2_9_38_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsnano.1c10680"},{"key":"e_1_2_9_39_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.nanoen.2023.108291"},{"key":"e_1_2_9_40_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.202106731"},{"key":"e_1_2_9_41_1","doi-asserted-by":"publisher","DOI":"10.1002\/aesr.202400301"},{"key":"e_1_2_9_42_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsaelm.4c01355"},{"key":"e_1_2_9_43_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.201202405"},{"key":"e_1_2_9_44_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202509631"},{"key":"e_1_2_9_45_1","doi-asserted-by":"publisher","DOI":"10.1016\/S0376\u20107388(00)80021\u20106"},{"key":"e_1_2_9_46_1","doi-asserted-by":"publisher","DOI":"10.1016\/S0376\u20107388(00)80020\u20104"},{"key":"e_1_2_9_47_1","doi-asserted-by":"publisher","DOI":"10.3390\/ijms232415757"},{"key":"e_1_2_9_48_1","doi-asserted-by":"publisher","DOI":"10.1007\/s42765\u2010025\u201000573\u20102"},{"key":"e_1_2_9_49_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.matt.2025.102155"},{"key":"e_1_2_9_50_1","doi-asserted-by":"crossref","first-page":"2016","DOI":"10.1007\/s42765-023-00316-1","article-title":"Plastic\u2010Swelling Preparation of Functional Graphene Aerogel Fiber Textiles","volume":"5","author":"Qi Y.","year":"2023","journal-title":"Advanced Fiber Materials"},{"key":"e_1_2_9_51_1","doi-asserted-by":"crossref","first-page":"4048","DOI":"10.3390\/polym13224048","article-title":"A Wet\u2010Spinning Process for Producing Carbon Nanotube\/Polyvinylidene Fluoride Fibers Having Highly Consistent Electrical and Mechanical Properties","volume":"13","author":"Kang K. 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