{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,9,17]],"date-time":"2026-09-17T06:04:27Z","timestamp":1789625067398,"version":"build-2803163510"},"reference-count":50,"publisher":"Wiley","license":[{"start":{"date-parts":[[2026,9,16]],"date-time":"2026-09-16T00:00:00Z","timestamp":1789516800000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/creativecommons.org\/licenses\/by\/4.0\/"},{"start":{"date-parts":[[2026,9,16]],"date-time":"2026-09-16T00:00:00Z","timestamp":1789516800000},"content-version":"tdm","delay-in-days":0,"URL":"http:\/\/doi.wiley.com\/10.1002\/tdm_license_1.1"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["22378105"],"award-info":[{"award-number":["22378105"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100004735","name":"Natural Science Foundation of Hunan Province","doi-asserted-by":"publisher","award":["2026JJ50007"],"award-info":[{"award-number":["2026JJ50007"]}],"id":[{"id":"10.13039\/501100004735","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["advanced.onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["Advanced Science"],"abstract":"<jats:title>ABSTRACT<\/jats:title>\n                  <jats:p>\n                    Engineering structurally defined interfacial motifs between isolated atoms and nanoparticles offers a promising route toward high\u2010performance electrocatalysis, yet achieving such motifs with clear structure\u2013function correlations remains difficult. Here, iridium (Ir) configurations comprising single atoms (SA), atomic\u2010layer patches (AL), and nanoparticles (NP) were constructed on tricopper phosphide nanowires as a model platform, yielding Ir\n                    <jats:sub>SA<\/jats:sub>\n                    \/Cu\n                    <jats:sub>3<\/jats:sub>\n                    P, Ir\n                    <jats:sub>AL<\/jats:sub>\n                    \/Cu\n                    <jats:sub>3<\/jats:sub>\n                    P, and Ir\n                    <jats:sub>NP<\/jats:sub>\n                    \/Cu\n                    <jats:sub>3<\/jats:sub>\n                    P, respectively. This configuration\u2010defined catalyst series reveals distinct structure\u2010dependent alkaline hydrogen evolution behavior. The atomic\u2010layer iridium patches exhibit a mixed\u2010valence interfacial state and anisotropic lattice distortion, as established by complementary microscopy, spectroscopy, and scattering analyses. Theory further reveals an edge\u2010to\u2010core charge gradient and indicates that this electronically graded interface optimizes Ir\n                    <jats:italic>5d<\/jats:italic>\n                    states to facilitate water dissociation and balance hydrogen adsorption\/desorption. Consequently, the iridium atomic\u2010layer catalyst achieves an overpotential of 27 mV at 10 mA cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    and reaches 1 A cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    at a cell voltage of 1.68 V in an anion exchange membrane electrolyzer. This work establishes mixed\u2010valence atomic\u2010layer metal patches as a functional platform for interfacial electrocatalysis.\n                  <\/jats:p>","DOI":"10.1002\/advs.77700","type":"journal-article","created":{"date-parts":[[2026,9,17]],"date-time":"2026-09-17T05:42:30Z","timestamp":1789623750000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Mixed\u2010Valence Atomic\u2010Layer Iridium Patches Enhance Alkaline Hydrogen Evolution"],"prefix":"10.1002","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-2535-3155","authenticated-orcid":false,"given":"Payam","family":"Ahmadian Koudakan","sequence":"first","affiliation":[{"name":"State Key Laboratory of Chemo and Biosensing College of Chemistry and Chemical Engineering and National Graduate College for Elite Engineers Hunan University  Changsha China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiaobin","family":"Hao","sequence":"additional","affiliation":[{"name":"School of Materials and Chemical Engineering Chuzhou University  Chuzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Rui","family":"Guo","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Chemo and Biosensing College of Chemistry and Chemical Engineering and National Graduate College for Elite Engineers Hunan University  Changsha China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9749-9842","authenticated-orcid":false,"given":"Omid","family":"Mazaheri","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Chemo and Biosensing College of Chemistry and Chemical Engineering and National Graduate College for Elite Engineers Hunan University  Changsha China"},{"name":"Department of Chemical Engineering The University of Melbourne  Parkville Victoria Australia"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0006-6426-3581","authenticated-orcid":false,"given":"Matthias","family":"Pichler","sequence":"additional","affiliation":[{"name":"Department of Chemical Engineering The University of Melbourne  Parkville Victoria Australia"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qinjian","family":"Luo","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Chemo and Biosensing College of Chemistry and Chemical Engineering and National Graduate College for Elite Engineers Hunan University  Changsha China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Bufeng","family":"Zhang","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Chemo and Biosensing College of Chemistry and Chemical Engineering and National Graduate College for Elite Engineers Hunan University  Changsha China"},{"name":"Hunan Provincial Polyimide Film Engineering Technology Research Center Zhuzhou Times Huaxin New Material Technology Co., Ltd. Zhuzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-6370-2470","authenticated-orcid":false,"given":"Shuaijun","family":"Pan","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Chemo and Biosensing College of Chemistry and Chemical Engineering and National Graduate College for Elite Engineers Hunan University  Changsha China"},{"name":"Department of Chemical Engineering The University of Melbourne  Parkville Victoria Australia"},{"name":"Hunan Provincial Polyimide Film Engineering Technology Research Center Zhuzhou Times Huaxin New Material Technology Co., Ltd. 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