{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,4]],"date-time":"2026-10-04T16:51:58Z","timestamp":1791132718976,"version":"4.1.0"},"reference-count":216,"publisher":"Wiley","license":[{"start":{"date-parts":[[2026,10,4]],"date-time":"2026-10-04T00:00:00Z","timestamp":1791072000000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/creativecommons.org\/licenses\/by\/4.0\/"},{"start":{"date-parts":[[2026,10,4]],"date-time":"2026-10-04T00:00:00Z","timestamp":1791072000000},"content-version":"tdm","delay-in-days":0,"URL":"http:\/\/doi.wiley.com\/10.1002\/tdm_license_1.1"}],"content-domain":{"domain":["advanced.onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["Advanced Science"],"abstract":"<jats:title>ABSTRACT<\/jats:title>\n                  <jats:p>The development of Pt\u2010free electrocatalysts is critical for reducing the cost of hydrogen production through the hydrogen evolution reaction (HER). Although extensive efforts have focused on improving the intrinsic activity of earth\u2010abundant catalysts, the role of the catalyst\u2013support interface remains comparatively underexplored. Carbon cloth (CC) has emerged as an attractive electrode platform owing to its electrical conductivity, hierarchical porosity, mechanical flexibility, chemical stability, and ability to facilitate efficient charge and mass transport. Although CC is generally not the primary HER active phase, it can strongly influence electrode\u2010level performance by regulating interfacial electron transfer, catalyst anchoring, active\u2010site accessibility, wettability, hydrogen bubble release, and long\u2010term durability. This review critically analyzes the interfacial synergy between CC and Pt\u2010free transition\u2010metal\u2010based catalysts, including Co\u2010, Ni\u2010, Fe\u2010, Cu\u2010, Mo\u2010, and W\u2010based systems, with and without heteroatom or anion modification involving N, P, and S species. The HER activity and stability of these systems are evaluated under acidic, alkaline, neutral, and pH\u2010universal conditions. A particular emphasis is placed on how catalyst\u2013support interactions, synthesis strategies, surface chemistry, structural features, and mass\u2010transport behavior collectively determine electrochemical performance. Finally, current challenges and future opportunities are discussed, including mechanistic understanding, operando characterization, high\u2010current\u2010density operation, long\u2010term durability, scalable fabrication, and practical electrolyzer integration.<\/jats:p>","DOI":"10.1002\/advs.77763","type":"journal-article","created":{"date-parts":[[2026,10,4]],"date-time":"2026-10-04T15:53:53Z","timestamp":1791129233000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Engineering Carbon Cloth\u2010Catalyst Interfaces for Pt\u2010Free Hydrogen Evolution Across the Full pH Spectrum"],"prefix":"10.1002","author":[{"ORCID":"https:\/\/orcid.org\/0009-0004-5779-5243","authenticated-orcid":false,"given":"Syed Mohammed","family":"Hubaish","sequence":"first","affiliation":[{"name":"Gas Processing Center (GPC) College of Engineering Qatar University  Doha Qatar"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8314-5752","authenticated-orcid":false,"given":"Belal","family":"Salah","sequence":"additional","affiliation":[{"name":"Gas Processing Center (GPC) College of Engineering Qatar University  Doha Qatar"},{"name":"Center for Advanced Materials Qatar University  Doha Qatar"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-5701-5957","authenticated-orcid":false,"given":"Khouloud","family":"Jlassi","sequence":"additional","affiliation":[{"name":"Center for Advanced Materials Qatar University  Doha Qatar"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-4270-6258","authenticated-orcid":false,"given":"Ali A.","family":"Abdelhafiz","sequence":"additional","affiliation":[{"name":"Department of Nuclear Science Engineering Massachusetts Institute of Technology  Cambridge Massachusetts USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-5327-2497","authenticated-orcid":false,"given":"Kamel","family":"Eid","sequence":"additional","affiliation":[{"name":"Gas Processing Center (GPC) College of Engineering Qatar University  Doha Qatar"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2026,10,4]]},"reference":[{"issue":"4","key":"e_1_2_17_2_1","doi-asserted-by":"crossref","first-page":"1276","DOI":"10.1039\/D2GC02748H","article-title":"Graphitic Carbon Nitride\u2010based Nanostructures as Emergent Catalysts for Carbon Monoxide (CO) Oxidation","volume":"25","author":"Eid K.","year":"2023","journal-title":"Green Chemistry"},{"issue":"17","key":"e_1_2_17_3_1","doi-asserted-by":"crossref","first-page":"6748","DOI":"10.1039\/D3GC01790G","article-title":"Scalable Nitrogen\u2010enriched Porous Sub\u2010100 Nm Graphitic Carbon Nanocapsules for Efficient Oxygen Reduction 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