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Precise control over their critical parameters is essential to enhance performance and expand the range of applications. In this work, we develop a cascaded third\u2010order nonlinear system to create an on\u2010demand and customized itinerant frequency comb (IFC). Unlike traditional microcavity Kerr combs, the IFC decouples the comb center frequency from the cavity resonance, thereby enabling arbitrary spectral width scaling and flexible comb spacing adjustments. In particular, we demonstrate the real\u2010time engineering of the central frequency of IFCs, thereby enabling the splicing and subdivision of frequency combs. These advances have the potential to enhance the performance of existing applications and expand new application scenarios by harnessing cascaded nonlinear\u00a0effects.<\/jats:p>","DOI":"10.1002\/advs.77903","type":"journal-article","created":{"date-parts":[[2026,9,27]],"date-time":"2026-09-27T18:00:31Z","timestamp":1790532031000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Customized Itinerant Frequency Combs by Cascaded Nonlinear Effects"],"prefix":"10.1002","author":[{"given":"Yi","family":"Wang","sequence":"first","affiliation":[{"name":"Beijing Key Laboratory of Fault\u2010Tolerant Quantum Computing Beijing Academy of Quantum Information Sciences Beijing China"},{"name":"Key Laboratory of Low\u2010Dimensional Quantum Structures and Quantum Control of Ministry of Education, Key Laboratory for Matter Microstructure and Function of Hunan Province, Department of Physics and Synergetic Innovation Center for 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