{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,4]],"date-time":"2026-10-04T15:53:11Z","timestamp":1791129191553,"version":"4.1.0"},"reference-count":72,"publisher":"Wiley","license":[{"start":{"date-parts":[[2026,10,4]],"date-time":"2026-10-04T00:00:00Z","timestamp":1791072000000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/creativecommons.org\/licenses\/by\/4.0\/"},{"start":{"date-parts":[[2026,10,4]],"date-time":"2026-10-04T00:00:00Z","timestamp":1791072000000},"content-version":"tdm","delay-in-days":0,"URL":"http:\/\/doi.wiley.com\/10.1002\/tdm_license_1.1"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["52373074"],"award-info":[{"award-number":["52373074"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100004543","name":"China Scholarship Council","doi-asserted-by":"publisher","award":["202408440282"],"award-info":[{"award-number":["202408440282"]}],"id":[{"id":"10.13039\/501100004543","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["advanced.onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["Advanced Science"],"abstract":"<jats:title>ABSTRACT<\/jats:title>\n                  <jats:p>\n                    Lithium metal batteries offer high energy density but suffer from severe safety risks associated with dendrite growth and flammable electrolytes, which can lead to thermal runaway and combustion. Although solid\u2010state electrolytes improve thermal stability, they primarily rely on intrinsic nonflammability and remain ineffective in suppressing combustion once thermal runaway is triggered. Here, we report a dual\u2010functional fire\u2010safe microcapsule\u2010enabled strategy to construct hierarchical solid polymer electrolytes (HSPEs) with integrated fire\u2010suppression capability. Fire\u2010extinguishing agents, perfluoro(2\u2010methyl\u20103\u2010pentanone), are encapsulated within ammonium hydrogen phytate\u2010modified urea\u2010formaldehyde\u2010based resin shells and incorporated into an ethylene\u2010vinyl acetate matrix. Upon thermal stimulation, the microcapsules undergo rapid structural rupture, releasing perfluoro(2\u2010methyl\u20103\u2010pentanone) to suppress combustion, while the ammonium hydrogen phytate\u2010derived shell forms a protective char layer that retards heat and mass transfer. This dual\u2010functional design enables thermally triggered fire suppression within the electrolyte framework. Importantly, the HSPEs maintain desirable electrochemical properties, including a room\u2010temperature ionic conductivity of 0.64\u00a0mS\u00a0cm\n                    <jats:sup>\u22121<\/jats:sup>\n                    and an electrochemical stability window of up to 4.6\u00a0V. Furthermore, pouch cells based on HSPEs effectively resist ignition under thermal abuse conditions. This work provides a viable approach to integrating fire\u2010suppression functionality into solid\u2010state electrolytes, offering new insights into the design of safer lithium metal batteries.\n                  <\/jats:p>","DOI":"10.1002\/advs.78034","type":"journal-article","created":{"date-parts":[[2026,10,4]],"date-time":"2026-10-04T15:43:09Z","timestamp":1791128589000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Fire\u2010Safe Hierarchical Solid Polymer Electrolytes Enabled by Dual\u2010Functional Microcapsules for Lithium Metal Batteries"],"prefix":"10.1002","author":[{"given":"Ziqi","family":"Huang","sequence":"first","affiliation":[{"name":"College of Materials and Chemical Engineering, Key Laboratory for Biobased Materials and Energy of Ministry of Education South China Agricultural University  Guangzhou People's Republic of China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jiuqing","family":"Gui","sequence":"additional","affiliation":[{"name":"College of Materials and Chemical Engineering, Key Laboratory for Biobased Materials and Energy of Ministry of Education South China Agricultural University  Guangzhou People's Republic of China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qiaoying","family":"Cao","sequence":"additional","affiliation":[{"name":"College of Materials and Chemical Engineering, Key Laboratory for Biobased Materials and Energy of Ministry of Education South China Agricultural University  Guangzhou People's Republic of China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yong","family":"Xiao","sequence":"additional","affiliation":[{"name":"College of Materials and Chemical Engineering, Key Laboratory for Biobased Materials and Energy of Ministry of Education South China Agricultural University  Guangzhou People's Republic of China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hang","family":"Hu","sequence":"additional","affiliation":[{"name":"College of Materials and Chemical Engineering, Key Laboratory for Biobased Materials and Energy of Ministry of Education South China Agricultural University  Guangzhou People's Republic of China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-6169-9981","authenticated-orcid":false,"given":"Yeru","family":"Liang","sequence":"additional","affiliation":[{"name":"College of Materials and Chemical Engineering, Key Laboratory for Biobased Materials and Energy of Ministry of Education South China Agricultural University  Guangzhou People's Republic of China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2026,10,4]]},"reference":[{"key":"e_1_2_8_2_1","doi-asserted-by":"crossref","first-page":"5793","DOI":"10.1016\/j.jma.2025.10.020","article-title":"Recent Advances in Magnesium and Magnesium Alloys for Next\u2010Generation High\u2010Energy\u2010Density Lithium Rechargeable Batteries","volume":"13","author":"Kim D. 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