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Inspired by its \u201cvine\u2010leaf\u201d system, we design a bionic cryogel that functionalizes daytime cooling and nighttime thermal buffering, promoting sustainable and comfortable housing and living environments. The aligned channels mimic vine tendrils, delivering an ultralow radial thermal conductivity (0.035\u00a0W m\n                    <jats:sup>\u22121<\/jats:sup>\n                    \u00b7K\n                    <jats:sup>\u22121<\/jats:sup>\n                    ), high solar reflectance (95.28%), and high infrared emissivity (97.04%). Embedded phase\u2010change materials (PCMs) present leaf\u2010like, functionalized structures that store excess solar energy during the daytime and release latent heat at night, achieving 6.2\u00b0C sub\u2010ambient cooling under sunlight. In darkness, the stored latent heat is released, keeping the cryogel 2.4\u00b0C above ambient and preventing nocturnal overcooling. This spatiotemporal synergy between daytime radiative cooling and nighttime heat release enables climate\u2010adaptive thermal management, reducing the urban heat buildup with no need for electricity consumption. Our bionic design shifts thermal regulation from passive adaptation to active thermal planning using low carbon footprint materials as proven by life cycle assessment (LCA), offering a more sustainable pathway for energy\u2010efficient buildings.\n                  <\/jats:p>","DOI":"10.1002\/advs.78323","type":"journal-article","created":{"date-parts":[[2026,10,16]],"date-time":"2026-10-16T03:19:00Z","timestamp":1792120740000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Biobased Boston Ivy\u2010Inspired Cryogel Integrating Radiative Cooling and Phase Change Energy Storage for Adaptive Thermal Regulation"],"prefix":"10.1002","author":[{"given":"Sining","family":"Huang","sequence":"first","affiliation":[{"name":"State Key Laboratory of Utilization of Woody Oil Resource Northeast Forestry University  Harbin People's Republic of China"},{"name":"Horticultural Branch Heilongjiang Academy of Agricultural Sciences  Harbin Heilongjiang People's Republic of China"},{"name":"Key Laboratory of Bio\u2010based Material Science &amp; Technology (Ministry of Education) Northeast Forestry University  Harbin People's Republic of China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-2455-5153","authenticated-orcid":false,"given":"Zhiguo","family":"Li","sequence":"additional","affiliation":[{"name":"Key Laboratory of Bio\u2010based Material Science &amp; Technology (Ministry of Education) Northeast Forestry University  Harbin People's Republic of China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-4745-4945","authenticated-orcid":false,"given":"Yang","family":"Liu","sequence":"additional","affiliation":[{"name":"Key Laboratory of Bio\u2010based Material Science &amp; Technology (Ministry of Education) Northeast Forestry University  Harbin People's Republic of 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