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However, this promising approach has proved challenging to inherit in all\u2010solid\u2010state Li metal batteries (ASSLMBs) because of the rigidity of inorganic solid electrolytes (SEs), which constrains interfacial solid\u2013solid ionic contact. Herein, a 3D Li anode is in situ constructed for ASSLMBs by spontaneous chemical reactions between halide SEs and Li metal. The in situ formed Li\u2013Al alloys and well\u2010maintained sulfide SEs inside the 3D structure serve as continuous electron and Li\n                    <jats:sup>+<\/jats:sup>\n                    transport pathways and facilitate the homogenous distribution of charge carriers. The lithiophilic Li alloy can regulate Li deposition behavior and enable uniform Li nucleation and deposition. Both the Li||Li symmetric and full batteries exhibit good electrochemical performance at high current density. This work provides a universal strategy and new insight perspective to construct 3D Li for high\u2010performance ASSLMBs.\n                  <\/jats:p>","DOI":"10.1002\/aenm.202300815","type":"journal-article","created":{"date-parts":[[2023,5,11]],"date-time":"2023-05-11T07:15:17Z","timestamp":1683789317000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":100,"title":["In Situ Constructed 3D Lithium Anodes for Long\u2010Cycling All\u2010Solid\u2010State Batteries"],"prefix":"10.1002","volume":"13","author":[{"given":"Hui","family":"Duan","sequence":"first","affiliation":[{"name":"Department of Mechanical and Materials Engineering University of Western Ontario  London Ontario N6A 5B9 Canada"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Changhong","family":"Wang","sequence":"additional","affiliation":[{"name":"Department of Mechanical and Materials Engineering University of Western Ontario  London Ontario N6A 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