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Herein, we reported an adaptive assembly strategy in dative B\u2190N framework, enabling dimension\u2010controlled synthesis of luminescent heterostructures with stimuli\u2010responsive properties. The conformational flexibility of boroxine units permit the epitaxial ligand to form the similar conformation as the seed ligand, triggering the adaptive hetero\u2010assembly between different frameworks. Moreover, the structural similarity on side chains of seed and epitaxial ligands determines the spatial matching degree at heterointerface, and thus adjusting the structural types of ligand side chains enables precise regulation of both the interfacial lattice matching and assembly orientation, thereby constructing one\u2010dimensional and two\u2010dimensional B\u2190N framework heterostructures. The resulting heterostructures exhibit spatially\u2010resolved stimuli\u2010responsive emission by inheriting intramolecular charge transfer of ligands, functioning as photonic barcode labels with multi\u2010level authentication capability. 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