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Herein, a novel ambient Li\u2010SO<jats:sub>2<\/jats:sub> battery was developed through the introduction of ionic liquid (IL) electrolytes with tailored basicities to solvate SO<jats:sub>2<\/jats:sub> by reversible chemical absorption. By tuning the interactions of ILs with SO<jats:sub>2<\/jats:sub>, a high energy density and good discharge performance with operating voltages above 2.8\u2005V were obtained. This strategy based on reversible chemical absorption of SO<jats:sub>2<\/jats:sub> in IL electrolytes enables the development of the next generation of ambient Li\u2010SO<jats:sub>2<\/jats:sub> batteries.<\/jats:p>","DOI":"10.1002\/anie.201309539","type":"journal-article","created":{"date-parts":[[2014,1,20]],"date-time":"2014-01-20T14:49:02Z","timestamp":1390229342000},"page":"2099-2103","source":"Crossref","is-referenced-by-count":69,"title":["Ambient Lithium\u2013SO<sub>2<\/sub> Batteries with Ionic Liquids as Electrolytes"],"prefix":"10.1002","volume":"53","author":[{"given":"Huabin","family":"Xing","sequence":"first","affiliation":[],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Chen","family":"Liao","sequence":"additional","affiliation":[],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Qiwei","family":"Yang","sequence":"additional","affiliation":[],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Gabriel 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