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For sour gas fields, selective and energy\u2010efficient removal of H<jats:sub>2<\/jats:sub>S is one of the crucial challenges facing the natural\u2010gas industry. Separation using nanoporous materials, such as zeolites, can be an alternative to energy\u2010intensive amine\u2010based absorption processes. Herein, the adsorption of binary H<jats:sub>2<\/jats:sub>S\/CH<jats:sub>4<\/jats:sub> and H<jats:sub>2<\/jats:sub>S\/C<jats:sub>2<\/jats:sub>H<jats:sub>6<\/jats:sub> mixtures in the all\u2010silica forms of 386\u2005zeolitic frameworks is investigated using Monte Carlo simulations. Adsorption of a five\u2010component mixture is utilized to evaluate the performance of the 16 most promising materials under close\u2010to\u2010real conditions. It is found that depending on the fractions of CH<jats:sub>4<\/jats:sub>, C<jats:sub>2<\/jats:sub>H<jats:sub>6<\/jats:sub>, and CO<jats:sub>2<\/jats:sub>, different sorbents allow for optimal H<jats:sub>2<\/jats:sub>S removal and hydrocarbon recovery.<\/jats:p>","DOI":"10.1002\/anie.201600612","type":"journal-article","created":{"date-parts":[[2016,4,18]],"date-time":"2016-04-18T07:20:00Z","timestamp":1460964000000},"page":"5938-5942","source":"Crossref","is-referenced-by-count":58,"title":["Identifying Optimal Zeolitic Sorbents for Sweetening of Highly Sour Natural Gas"],"prefix":"10.1002","volume":"55","author":[{"ORCID":"https:\/\/orcid.org\/0000-0001-5255-6922","authenticated-orcid":false,"given":"Mansi S.","family":"Shah","sequence":"first","affiliation":[{"name":"Department of Chemical Engineering and Materials Science University of Minnesota  421 Washington Avenue SE Minneapolis MN 55455-0132 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Michael","family":"Tsapatsis","sequence":"additional","affiliation":[{"name":"Department of Chemical Engineering and Materials Science University of Minnesota  421 Washington Avenue SE Minneapolis MN 55455-0132 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"J. 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