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Developing strategies that can simultaneously convert both CO<jats:sub>2<\/jats:sub> and H<jats:sub>2<\/jats:sub>S into value\u2010added products is attractive; however it has not received enough attention. A solar\u2010driven electrochemical process is demonstrated using graphene\u2010encapsulated zinc oxide catalyst for CO<jats:sub>2<\/jats:sub> reduction and graphene catalyst for H<jats:sub>2<\/jats:sub>S oxidation mediated by EDTA\u2010Fe<jats:sup>2+<\/jats:sup>\/EDTA\u2010Fe<jats:sup>3+<\/jats:sup> redox couples. The as\u2010prepared solar\u2010driven electrochemical system can realize the simultaneous conversion of CO<jats:sub>2<\/jats:sub> and H<jats:sub>2<\/jats:sub>S into carbon monoxide and elemental sulfur at near neutral conditions with high stability and selectivity. This conceptually provides an alternative avenue for the purification of natural gas with added economic and environmental benefits.<\/jats:p>","DOI":"10.1002\/anie.201713029","type":"journal-article","created":{"date-parts":[[2018,2,7]],"date-time":"2018-02-07T07:22:42Z","timestamp":1517988162000},"page":"3473-3477","source":"Crossref","is-referenced-by-count":89,"title":["Achieving Simultaneous CO<sub>2<\/sub> and H<sub>2<\/sub>S Conversion via a Coupled Solar\u2010Driven Electrochemical Approach on Non\u2010Precious\u2010Metal Catalysts"],"prefix":"10.1002","volume":"57","author":[{"given":"Weiguang","family":"Ma","sequence":"first","affiliation":[{"name":"State Key Laboratory of Catalysis Dalian Institute of Chemical Physics Chinese Academy of Sciences Dalian National Laboratory for Clean Energy, The Collaborative Innovation Center of Chemistry for Energy Materials (iChEM)  Zhongshan Road 457 Dalian 116023 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hong","family":"Wang","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Catalysis Dalian Institute of Chemical Physics Chinese Academy of Sciences Dalian National Laboratory for Clean Energy, The Collaborative Innovation Center of Chemistry for Energy Materials (iChEM)  Zhongshan Road 457 Dalian 116023 China"},{"name":"University of Chinese Academy of Sciences  Beijing 100049 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Wei","family":"Yu","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Catalysis Dalian Institute of Chemical Physics Chinese Academy of Sciences Dalian National Laboratory for Clean Energy, The Collaborative Innovation Center of Chemistry for Energy Materials (iChEM)  Zhongshan Road 457 Dalian 116023 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiaomei","family":"Wang","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Catalysis Dalian Institute of Chemical Physics Chinese Academy of Sciences Dalian National Laboratory for Clean Energy, The Collaborative Innovation Center of Chemistry for Energy Materials (iChEM)  Zhongshan Road 457 Dalian 116023 China"},{"name":"University of Chinese Academy of Sciences  Beijing 100049 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhiqiang","family":"Xu","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Catalysis Dalian Institute of Chemical Physics Chinese Academy of Sciences Dalian National Laboratory for Clean Energy, The Collaborative Innovation Center of Chemistry for Energy Materials (iChEM)  Zhongshan Road 457 Dalian 116023 China"},{"name":"University of Chinese Academy of Sciences  Beijing 100049 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xu","family":"Zong","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Catalysis Dalian Institute of Chemical Physics Chinese Academy of Sciences Dalian National Laboratory for Clean Energy, The Collaborative Innovation Center of Chemistry for Energy Materials (iChEM)  Zhongshan Road 457 Dalian 116023 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9301-7850","authenticated-orcid":false,"given":"Can","family":"Li","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Catalysis Dalian Institute of Chemical Physics Chinese Academy of Sciences Dalian National Laboratory for Clean Energy, The Collaborative Innovation Center of Chemistry for Energy Materials (iChEM)  Zhongshan Road 457 Dalian 116023 China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2018,2,27]]},"reference":[{"key":"e_1_2_2_1_1","first-page":"22","volume":"31","author":"Yu Y.","year":"2011","journal-title":"Nat. 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