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This has been utilized in light sources, displays, bioimaging, and advanced sensors. Organic ML materials are strongly limited to application by in\u2005situ unrepeatable ML. Now, in\u2005situ solar\u2010renewable organic ML materials can be formed by introducing a soft alkyl chain into an ML unit. For the first time, the ML from these polycrystalline thin films can be iteratively produced by simply recrystallizing the fractured crystal in\u2005situ after a contactless exposure to sunlight within a short time (\u226460\u2005s). Additionally, their ML color and lifetime can be also easily tuned by doping with organic luminescent dyes. Therefore, large\u2010area sandwich\u2010type organic ML devices can be fabricated, which can be repeatedly used in a colorful piezo\u2010display, visual handwriting monitor, and sensitive optical sensor, showing a lowest pressure threshold for ML of about 5\u2005kPa.<\/jats:p>","DOI":"10.1002\/anie.201806861","type":"journal-article","created":{"date-parts":[[2018,8,10]],"date-time":"2018-08-10T03:44:43Z","timestamp":1533872683000},"page":"12727-12732","update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":145,"title":["Alkyl Chain Introduction: In\u2005Situ Solar\u2010Renewable Colorful Organic Mechanoluminescence Materials"],"prefix":"10.1002","volume":"57","author":[{"given":"Wenlang","family":"Li","sequence":"first","affiliation":[{"name":"PCFM Lab, GDHPPC Lab Guangdong Engineering Technology Research Center for High-performance Organic and Polymer Photoelectric Functional Films State Key Laboratory of OEMT School of Chemistry 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