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The nanoscale surface arrangement of both photo\u2010 and electrochemically\u2010active components is essential for the function of the thin films. Layers of well\u2010defined ruthenium complexes on indium\u2010tin\u2010oxide electrodes provide electron\u2010transport channels that allow the electrochemical addressing of layers of isostructural cobalt complexes. These cobalt complexes are electrochemically inactive when assembled directly on transparent metal\u2010oxide electrodes. The interlayer of ruthenium complexes on such electrodes allows irreversible oxidation of the cobalt complexes. However, shifting the redox properties of the ruthenium complexes by excitation with light opens up an electron\u2010transport channel to reduce the cobalt complexes; hence releasing the trapped positive charges.<\/jats:p>","DOI":"10.1002\/anie.201807453","type":"journal-article","created":{"date-parts":[[2018,7,25]],"date-time":"2018-07-25T10:10:36Z","timestamp":1532513436000},"page":"13459-13464","update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":10,"title":["Light\u2010Triggered Release of Trapped Charges in Molecular Assemblies"],"prefix":"10.1002","volume":"57","author":[{"given":"Renata","family":"Balgley","sequence":"first","affiliation":[{"name":"Department of Organic Chemistry The Weizmann Institute of Science  7610001 Rehovot Israel"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Yadid M.","family":"Algavi","sequence":"additional","affiliation":[{"name":"Department of Organic Chemistry The Weizmann Institute of Science  7610001 Rehovot Israel"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Neta","family":"Elool\u2005Dov","sequence":"additional","affiliation":[{"name":"Department of Organic Chemistry The Weizmann Institute of Science  7610001 Rehovot Israel"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-4831-221X","authenticated-orcid":false,"given":"Michal","family":"Lahav","sequence":"additional","affiliation":[{"name":"Department of Organic Chemistry The Weizmann Institute of Science  7610001 Rehovot Israel"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-4102-4220","authenticated-orcid":false,"given":"Milko E.","family":"van\u2005der\u2005Boom","sequence":"additional","affiliation":[{"name":"Department of Organic Chemistry The Weizmann Institute of Science  7610001 Rehovot Israel"}],"role":[{"role":"author","vocabulary":"crossref"}]}],"member":"311","published-online":{"date-parts":[[2018,8,15]]},"reference":[{"key":"e_1_2_2_1_1","first-page":"449","volume-title":"Principles of Neural Science","author":"Kandel E. 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