{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,9]],"date-time":"2026-10-09T10:00:48Z","timestamp":1791540048136,"version":"4.3.4"},"reference-count":29,"publisher":"Wiley","issue":"7","license":[{"start":{"date-parts":[[2019,1,3]],"date-time":"2019-01-03T00:00:00Z","timestamp":1546473600000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/onlinelibrary.wiley.com\/termsAndConditions#vor"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["51872003, 51572003"],"award-info":[{"award-number":["51872003, 51572003"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["Angew Chem Int Ed"],"published-print":{"date-parts":[[2019,2,11]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>\n                    A rapid and highly efficient strategy for introducing C into g\u2010C\n                    <jats:sub>3<\/jats:sub>\n                    N\n                    <jats:sub>4<\/jats:sub>\n                    involves copolymerizing \u03c0\u2010electron\u2010rich barbituric acid with melamine via a facile microwave\u2010assisted heating, thereby eliminating the issues in conventional electric furnace heating, such as the severe volatilization, owing to the mismatch of the sublimation temperatures of barbituric acid and melamine. The g\u2010C\n                    <jats:sub>3<\/jats:sub>\n                    N\n                    <jats:sub>4<\/jats:sub>\n                    catalyst after optimizing the C\u2010doping content actively generates increased amounts of H\n                    <jats:sub>2<\/jats:sub>\n                    under visible light exposure with the highest H\n                    <jats:sub>2<\/jats:sub>\n                    generation rate of 25.0\u2005\u03bcmol\u2009h\n                    <jats:sup>\u22121<\/jats:sup>\n                    , which is nearly 20 times above that using g\u2010C\n                    <jats:sub>3<\/jats:sub>\n                    N\n                    <jats:sub>4<\/jats:sub>\n                    produced by conventional electric furnace heating of two identical monomers (1.3\u2005\u03bcmol\u2009h\n                    <jats:sup>\u22121<\/jats:sup>\n                    ). As such, the microwave\u2010assisted heating strategy may stand out as an extremely simple route to incorporating \u03c0\u2010electrons into g\u2010C\n                    <jats:sub>3<\/jats:sub>\n                    N\n                    <jats:sub>4<\/jats:sub>\n                    with markedly improved photocatalytic performance.\n                  <\/jats:p>","DOI":"10.1002\/anie.201813117","type":"journal-article","created":{"date-parts":[[2018,12,7]],"date-time":"2018-12-07T12:45:52Z","timestamp":1544186752000},"page":"1985-1989","update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":269,"title":["Achieving Efficient Incorporation of \u03c0\u2010Electrons into Graphitic Carbon Nitride for Markedly Improved Hydrogen Generation"],"prefix":"10.1002","volume":"58","author":[{"given":"Jing","family":"Li","sequence":"first","affiliation":[{"name":"School of Chemistry and Chemical Engineering Anhui Province Key Laboratory of Chemistry for Inorganic\/Organic Hybrid Functionalized Materials Institute of Physical Science and Information Technology Anhui University  Hefei 230601 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Dandan","family":"Wu","sequence":"additional","affiliation":[{"name":"School of Chemistry and Chemical Engineering Anhui Province Key Laboratory of Chemistry for Inorganic\/Organic Hybrid Functionalized Materials Institute of Physical Science and Information Technology Anhui University  Hefei 230601 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"James","family":"Iocozzia","sequence":"additional","affiliation":[{"name":"School of Materials Science and Engineering Georgia Institute of Technology  Atlanta GA 30332 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Haiwei","family":"Du","sequence":"additional","affiliation":[{"name":"School of Chemistry and Chemical Engineering Anhui Province Key Laboratory of Chemistry for Inorganic\/Organic Hybrid Functionalized Materials Institute of Physical Science and Information Technology Anhui University  Hefei 230601 P. R. 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China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhen","family":"Li","sequence":"additional","affiliation":[{"name":"Faculty of Materials Science and Chemistry China University of Geoscience (Wuhan)  Wuhan 430074 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhaoming","family":"Xue","sequence":"additional","affiliation":[{"name":"School of Chemistry and Chemical Engineering Anhui Province Key Laboratory of Chemistry for Inorganic\/Organic Hybrid Functionalized Materials Institute of Physical Science and Information Technology Anhui University  Hefei 230601 P. R. 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