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We report here the facile synthesis of monodisperse polymer nanocapsules via a redox\u2010mediated kinetic strategy from two simple molecules: dopamine and benzene\u20101,4\u2010dithiol (BDT). Specifically, BDT forms core templates and modulates the oxidation kinetics of dopamine into polydopamine (PDA) shells. These uniform nanoparticles can be tuned between \u224870 and 200\u2005nm because the core diameter directly depends on BDT while the shell thickness depends on dopamine. The supramolecular core can then rapidly disassemble in organic solvents to produce PDA nanocapsules. Such nanocapsules exhibit enhanced physicochemical performance (e.g., loading capacity, photothermal transduction, and anti\u2010oxidation) versus their solid counterparts. 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