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However, organic molecules with high potential are rare, and the voltage of most reported organic cathode\u2010based ZIBs is less than 1.2\u2005V. Herein, we explored the redox process of p\u2010type organics and figured out the relationship between energy change and voltage output during the process. Then, we proposed a dual\u2010step strategy to effectively tune the energy change and eventually improve the output voltage of the organic electrode. Combining the regulation of the electron cloud of organic molecules and the manipulation of the solvation structure, the output voltage of an organosulfur compound based ZIB was greatly increased from 0.8\u2005V to 1.7\u2005V. Our results put forward a specific pathway to improve the working voltage and lay the foundation for the practical application of organic electrodes.<\/jats:p>","DOI":"10.1002\/anie.202203453","type":"journal-article","created":{"date-parts":[[2022,5,9]],"date-time":"2022-05-09T10:38:56Z","timestamp":1652092736000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":160,"title":["High\u2010Voltage Organic Cathodes for Zinc\u2010Ion Batteries through Electron Cloud and Solvation Structure Regulation"],"prefix":"10.1002","volume":"61","author":[{"given":"Huilin","family":"Cui","sequence":"first","affiliation":[{"name":"Department of Materials Science and Engineering City University of Hong Kong  83 Tat Chee Avenue Kowloon 999077 Hong Kong"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Tairan","family":"Wang","sequence":"additional","affiliation":[{"name":"Department of Materials Science and Engineering City University of Hong Kong  83 Tat Chee Avenue Kowloon 999077 Hong Kong"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhaodong","family":"Huang","sequence":"additional","affiliation":[{"name":"Department of Materials Science and Engineering City University of Hong Kong  83 Tat Chee Avenue Kowloon 999077 Hong Kong"},{"name":"Hong Kong Center for Cerebro-Cardiovascular Health Engineering (COCHE)  Shatin, NT, HKSAR China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Guojin","family":"Liang","sequence":"additional","affiliation":[{"name":"Department of Materials Science and Engineering City University of Hong Kong  83 Tat Chee Avenue Kowloon 999077 Hong Kong"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ze","family":"Chen","sequence":"additional","affiliation":[{"name":"Department of Materials Science and Engineering City University of Hong Kong  83 Tat Chee Avenue Kowloon 999077 Hong Kong"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ao","family":"Chen","sequence":"additional","affiliation":[{"name":"Department of Materials Science and Engineering City University of Hong Kong  83 Tat Chee Avenue Kowloon 999077 Hong Kong"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Donghong","family":"Wang","sequence":"additional","affiliation":[{"name":"Department of Materials Science and Engineering City University of Hong Kong  83 Tat Chee Avenue Kowloon 999077 Hong Kong"},{"name":"Hong Kong Center for Cerebro-Cardiovascular Health Engineering (COCHE)  Shatin, NT, HKSAR China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qi","family":"Yang","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Chemical Resource Engineering College of Chemical Engineering Beijing University of Chemical Technology  Beijing 100029 P. 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